中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Effect Of SO2 on the performance of Ag-Pd/Al2O3 for the selective catalytic reduction of NOx with C2H5OH

文献类型:期刊论文

作者Xie Shu-xia; Yu Yun-bo; Wang Jin; He Hong
刊名JOURNAL OF ENVIRONMENTAL SCIENCES-CHINA
出版日期2006
卷号18期号:5页码:973-978
关键词sulphate SCR nitrate enolic species isocyanate reaction mechanism
英文摘要The influence of SO, on the performance of Ag-Pd/Al2O3 for the selective catalytic reduction (SCR) of NOx with C2H5OH was investigated experimentally. The activity test results suggest that Ag-Pd/Al2O3 shows a small activity loss in the presence Of SO2 when using C2H5OH as a reductant. In situ DRIFTS spectra show that the activity loss originates from the formation of surface sulphate species on the Ag-Pd/Al2O3. The surface sulphate species formation inhibits the formation of nitrate, whereas hardly changes the partial oxidation Of C2H5OH. Compared with the NOx reduction by C3H6 an obvious suppression of the surface sulphate species formation was observed by DRIFTS experiment when using C2H5OH as a reductant. This phenomenon reveals the better catalytic performance and strong SO2 tolerance ofAg-Pd/Al2O3-C2H5OH system.
WOS记录号WOS:000240445400024
源URL[http://ir.rcees.ac.cn/handle/311016/22873]  
专题生态环境研究中心_环境化学与生态毒理学国家重点实验室
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GB/T 7714
Xie Shu-xia,Yu Yun-bo,Wang Jin,et al. Effect Of SO2 on the performance of Ag-Pd/Al2O3 for the selective catalytic reduction of NOx with C2H5OH[J]. JOURNAL OF ENVIRONMENTAL SCIENCES-CHINA,2006,18(5):973-978.
APA Xie Shu-xia,Yu Yun-bo,Wang Jin,&He Hong.(2006).Effect Of SO2 on the performance of Ag-Pd/Al2O3 for the selective catalytic reduction of NOx with C2H5OH.JOURNAL OF ENVIRONMENTAL SCIENCES-CHINA,18(5),973-978.
MLA Xie Shu-xia,et al."Effect Of SO2 on the performance of Ag-Pd/Al2O3 for the selective catalytic reduction of NOx with C2H5OH".JOURNAL OF ENVIRONMENTAL SCIENCES-CHINA 18.5(2006):973-978.

入库方式: OAI收割

来源:生态环境研究中心

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