Carbon-doped anatase TiO2 nanotube array/glass and its enhanced photocatalytic activity under solar light
文献类型：期刊论文
| 作者 | Zhao, Yun1 ; Li, Yan1; Wang CW(王成伟)1,2; Wang, Jian1; Wang, Xiang-Qian1; Pan, Zi-Wei1; Dong, Chen1; Zhou F(周峰)2
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| 刊名 | Solid State Sciences
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| 出版日期 | 2013 |
| 卷号 | 15页码:53-59 |
| 关键词 | Anatase TiO2 nanotube arrays Carbon-doped Photocatalytic activity Simulated solar light |
| ISSN号 | 1293-2558 |
| 通讯作者 | 王成伟 |
| 英文摘要 | To enhance the photocatalytic activity under solar light, highly ordered TiO2 nanotube arrays (TNAs) film with anatase phase was fabricated on glass and successfully doped with carbon at various temperatures of 450-550 ℃. The characterization results indicate that, after carbon doping, the TNAs still remained nanotubular structure with anatase phase. But their optical response shifted from UV to the visible light region and the recombination of photogenerated carriers was suppressed effectively. It is more important that the carbon-doped TNAs/glass (C-TNAs) samples exhibited high solar light photocatalytic activity, and 68%, 61% and 56% MO was photodegraded in 150 min by the C-TNAs calcined at 550, 500 and 450 ℃, respectively. Especially, the apparent reaction rate constant of C-TNAs calcined at 550 (k, 0.065 min-1) with the highest activity is 3.6 times that of pristine anatase TNAs (k, 0.018 min-1). It is clear that carbon doping enhanced the photocatalytic activity under sunlight at optimized annealing temperature. The efficient activity could be attributed to the synergetic effects of strong visible light absorption, good crystallization, large surface, and enhanced separation of photoinduced carriers. |
| 学科主题 | 材料科学与物理化学 |
| 收录类别 | SCI |
| 资助信息 | the National Natural Science Foundation of China (Grant Nos. 10774121;10974155;11264034);the Foundation of Key Laboratory of Polymer Materials of Gansu Province (Grant No. KF-09-02);the Foundation of Northwest Normal University of China (Grant No. NWNU-LKQN-10-26) |
| 语种 | 英语 |
| WOS记录号 | WOS:000315070700009 |
| 源URL | [http://210.77.64.217/handle/362003/18243]  |
| 专题 | 兰州化学物理研究所_固体润滑国家重点实验室 |
| 作者单位 | 1.NW Normal Univ, Coll Phys & Elect Engn, Key Lab Atom & Mol Phys & Funct Mat Gansu Prov, Lanzhou 730070, Gansu, Peoples R China 2.Chinese Acad Sci, Lanzhou Inst Chem Phys, State Key Lab Solid Lubricat, Lanzhou 730000, Gansu, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhao, Yun,Li, Yan,Wang CW,et al. Carbon-doped anatase TiO2 nanotube array/glass and its enhanced photocatalytic activity under solar light[J]. Solid State Sciences,2013,15:53-59. |
| APA | Zhao, Yun.,Li, Yan.,Wang CW.,Wang, Jian.,Wang, Xiang-Qian.,...&Zhou F.(2013).Carbon-doped anatase TiO2 nanotube array/glass and its enhanced photocatalytic activity under solar light.Solid State Sciences,15,53-59. |
| MLA | Zhao, Yun,et al."Carbon-doped anatase TiO2 nanotube array/glass and its enhanced photocatalytic activity under solar light".Solid State Sciences 15(2013):53-59. |
入库方式： OAI收割
来源：兰州化学物理研究所
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