Catalytic wet oxidation of aqueous methylamine: comparative study on the catalytic performance of platinum-ruthenium, platinum, and ruthenium catalysts supported on titania
文献类型：期刊论文
| 作者 | Song AY(宋爱英)1,2,3; Lu GX(吕功煊)1
|
| 刊名 | Environmental Technology
 |
| 出版日期 | 2015 |
| 卷号 | 36期号:9页码:1160-1166 |
| 关键词 | methylamine Pt-Ru CWAO dispersion TiO2 |
| ISSN号 | 0959-3330 |
| 通讯作者 | 吕功煊 |
| 英文摘要 | Promotion of the dispersion of Ru species supported on TiO2 was achieved by introduction of Pt component and the role of Pt in enhancing the catalytic performances of Pt–Ru was investigated with catalytic wet air oxidation of methylamine used as a probing reaction. It was found that Pt–Ru/TiO2 displayed a much better catalytic performance compared with Pt/TiO2 and Ru/TiO2 catalysts due to having the highest dispersion of active species. Both high total organic carbon conversion and nitrogen selectivity (∼100%) over Pt–Ru/TiO2 catalyst were achieved at low temperature (200 °C). X-ray photoelectron spectroscopy characterization indicated that there were strong interactions between metal particles and the support, which may increase the catalytic performance of catalysts. |
| 学科主题 | 物理化学与绿色催化 |
| 收录类别 | SCI |
| 资助信息 | the National Science Foundation of China (Grant Nos.21373245;21173242);973 and 863 Program of Department of Sciences and Technology of China (Grant Nos. 2013CB632404;2012AA051501;2009CB22003);Gansu Provincial Science & Technology Department (1304FKCA085) |
| 语种 | 英语 |
| WOS记录号 | WOS:000350039900011 |
| 源URL | [http://210.77.64.217/handle/362003/19304]  |
| 专题 | 兰州化学物理研究所_OSSO国家重点实验室 兰州化学物理研究所_ERC国家工程研究中心 |
| 作者单位 | 1.Univ Chinese Acad Sci, Lanzhou Inst Chem Phys, State Key Lab Oxo Synth & Select Oxidat, Lanzhou 730000, Peoples R China 2.Gansu Inst Polit Sci & Law, Coll Publ Secur Technol, Lanzhou 730070, Peoples R China 3.Phys Chem Lab Gansu Prov Ctr Dis Control & Preven, Lanzhou 730020, Peoples R China |
| 推荐引用方式 GB/T 7714 | Song AY,Lu GX. Catalytic wet oxidation of aqueous methylamine: comparative study on the catalytic performance of platinum-ruthenium, platinum, and ruthenium catalysts supported on titania[J]. Environmental Technology,2015,36(9):1160-1166. |
| APA | Song AY,&Lu GX.(2015).Catalytic wet oxidation of aqueous methylamine: comparative study on the catalytic performance of platinum-ruthenium, platinum, and ruthenium catalysts supported on titania.Environmental Technology,36(9),1160-1166. |
| MLA | Song AY,et al."Catalytic wet oxidation of aqueous methylamine: comparative study on the catalytic performance of platinum-ruthenium, platinum, and ruthenium catalysts supported on titania".Environmental Technology 36.9(2015):1160-1166. |
入库方式： OAI收割
来源：兰州化学物理研究所
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