The structural origin of the hard-sphere glass transition in granular packing
文献类型:期刊论文
作者 | Xia, CJ; Li, JD; Cao, YX; Kou, BQ; Xiao, XH; Fezzaa, K; Xiao, TQ; Wang, YJ |
刊名 | NATURE COMMUNICATIONS
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出版日期 | 2015 |
卷号 | 6页码:— |
关键词 | FORMING LIQUIDS SUPERCOOLED LIQUIDS ORIENTATIONAL ORDER JAMMING TRANSITION LENGTH SCALES DYNAMICS RELAXATION REGIONS |
ISSN号 | 2041-1723 |
通讯作者 | Wang, YJ (reprint author), Shanghai Jiao Tong Univ, Dept Phys & Astron, 800 Dong Chuan Rd, Shanghai 200240, Peoples R China. |
英文摘要 | Glass transition is accompanied by a rapid growth of the structural relaxation time and a concomitant decrease of configurational entropy. It remains unclear whether the transition has a thermodynamic origin, and whether the dynamic arrest is associated with the growth of a certain static order. Using granular packing as a model hard-sphere glass, we show the glass transition as a thermodynamic phase transition with a 'hidden' polytetrahedral order. This polytetrahedral order is spatially correlated with the slow dynamics. It is geometrically frustrated and has a peculiar fractal dimension. Additionally, as the packing fraction increases, its growth follows an entropy-driven nucleation process, similar to that of the random first-order transition theory. Our study essentially identifies a long-sought-after structural glass order in hard-sphere glasses. |
语种 | 英语 |
WOS记录号 | WOS:000363138400001 |
公开日期 | 2016-03-08 |
源URL | [http://ir.sinap.ac.cn/handle/331007/25076] ![]() |
专题 | 上海应用物理研究所_中科院上海应用物理研究所2011-2017年 |
推荐引用方式 GB/T 7714 | Xia, CJ,Li, JD,Cao, YX,et al. The structural origin of the hard-sphere glass transition in granular packing[J]. NATURE COMMUNICATIONS,2015,6:—. |
APA | Xia, CJ.,Li, JD.,Cao, YX.,Kou, BQ.,Xiao, XH.,...&Wang, YJ.(2015).The structural origin of the hard-sphere glass transition in granular packing.NATURE COMMUNICATIONS,6,—. |
MLA | Xia, CJ,et al."The structural origin of the hard-sphere glass transition in granular packing".NATURE COMMUNICATIONS 6(2015):—. |
入库方式: OAI收割
来源:上海应用物理研究所
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