中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
The structural origin of the hard-sphere glass transition in granular packing

文献类型:期刊论文

作者Xia, CJ; Li, JD; Cao, YX; Kou, BQ; Xiao, XH; Fezzaa, K; Xiao, TQ; Wang, YJ
刊名NATURE COMMUNICATIONS
出版日期2015
卷号6页码:
关键词FORMING LIQUIDS SUPERCOOLED LIQUIDS ORIENTATIONAL ORDER JAMMING TRANSITION LENGTH SCALES DYNAMICS RELAXATION REGIONS
ISSN号2041-1723
通讯作者Wang, YJ (reprint author), Shanghai Jiao Tong Univ, Dept Phys & Astron, 800 Dong Chuan Rd, Shanghai 200240, Peoples R China.
英文摘要Glass transition is accompanied by a rapid growth of the structural relaxation time and a concomitant decrease of configurational entropy. It remains unclear whether the transition has a thermodynamic origin, and whether the dynamic arrest is associated with the growth of a certain static order. Using granular packing as a model hard-sphere glass, we show the glass transition as a thermodynamic phase transition with a 'hidden' polytetrahedral order. This polytetrahedral order is spatially correlated with the slow dynamics. It is geometrically frustrated and has a peculiar fractal dimension. Additionally, as the packing fraction increases, its growth follows an entropy-driven nucleation process, similar to that of the random first-order transition theory. Our study essentially identifies a long-sought-after structural glass order in hard-sphere glasses.
语种英语
WOS记录号WOS:000363138400001
公开日期2016-03-08
源URL[http://ir.sinap.ac.cn/handle/331007/25076]  
专题上海应用物理研究所_中科院上海应用物理研究所2011-2017年
推荐引用方式
GB/T 7714
Xia, CJ,Li, JD,Cao, YX,et al. The structural origin of the hard-sphere glass transition in granular packing[J]. NATURE COMMUNICATIONS,2015,6:—.
APA Xia, CJ.,Li, JD.,Cao, YX.,Kou, BQ.,Xiao, XH.,...&Wang, YJ.(2015).The structural origin of the hard-sphere glass transition in granular packing.NATURE COMMUNICATIONS,6,—.
MLA Xia, CJ,et al."The structural origin of the hard-sphere glass transition in granular packing".NATURE COMMUNICATIONS 6(2015):—.

入库方式: OAI收割

来源:上海应用物理研究所

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