中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Effect of aluminium dust on secondary organic aerosol formation in m-xylene/NOx photo-oxidation

文献类型:期刊论文

作者Liu Chang; Ma QingXin; Chu BiWu; Liu YongChun; He Hong; Zhang XiaoYe; Li JunHua; Hao JiMing
刊名SCIENCE CHINA-EARTH SCIENCES
出版日期2015-02
卷号58期号:2页码:245-254
关键词aromatic hydrocarbon m-xylene aluminium SOA aerosol size smog chamber
英文摘要As an important anthropogenic volatile organic compound (VOC), m-xylene has attracted numerous attentions due to its potential in secondary organic aerosol (SOA) formation. In this study, effects of aluminium dust seeds (boehmite and alumina) on SOA yield and aerosol size in m-xylene/NOx photo-oxidation were investigated in a 2 m(3) smog chamber at 30 degrees C and 50% relative humidity. Compared to the seed-free system, the presence of aluminium seeds resulted in an increase in the SOA yield, and also enhanced the O-3 concentration in the chamber. The photolysis of O-3 is a major source of OH radical, which is the most important oxidant of m-xylene. The increase in O-3 concentration could result in the generation of more OH radicals, and finally contribute to the SOA formation. Seed particles influence the SOA size mainly by acting as condensation nuclei. Semi-volatile organic compounds (SVOCs) were condensed onto these nuclei, resulting in the increase in SOA size. However, when aluminium seeds with high concentrations were introduced into the system, SVOCs that had been condensed onto each particle were dispersed by these seeds, leading to the reduction in aerosol size.
研究领域[WOS]Geosciences, Multidisciplinary
WOS记录号WOS:000348120900007
公开日期2016-03-15
源URL[http://ir.rcees.ac.cn/handle/311016/32469]  
专题生态环境研究中心_大气污染控制中心
推荐引用方式
GB/T 7714
Liu Chang,Ma QingXin,Chu BiWu,et al. Effect of aluminium dust on secondary organic aerosol formation in m-xylene/NOx photo-oxidation[J]. SCIENCE CHINA-EARTH SCIENCES,2015,58(2):245-254.
APA Liu Chang.,Ma QingXin.,Chu BiWu.,Liu YongChun.,He Hong.,...&Hao JiMing.(2015).Effect of aluminium dust on secondary organic aerosol formation in m-xylene/NOx photo-oxidation.SCIENCE CHINA-EARTH SCIENCES,58(2),245-254.
MLA Liu Chang,et al."Effect of aluminium dust on secondary organic aerosol formation in m-xylene/NOx photo-oxidation".SCIENCE CHINA-EARTH SCIENCES 58.2(2015):245-254.

入库方式: OAI收割

来源:生态环境研究中心

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