Occurrence of Synthetic Phenolic Antioxidants and Major Metabolites in Municipal Sewage Sludge in China
文献类型：期刊论文
| 作者 | Liu, Runzeng; Song, Shanjun; Lin, Yongfeng; Ruan, Ting; Jiang, Guibin |
| 刊名 | ENVIRONMENTAL SCIENCE & TECHNOLOGY
 |
| 出版日期 | 2015-02-17 |
| 卷号 | 49期号:4页码:2073-2080 |
| 英文摘要 | Synthetic phenolic antioxidants (SPAs) are one group of widely used additive chemicals, which have not yet had focused attention except for a few compounds such as 2,6-di-tert-butyl-4-methylphenol (BHT). In this study, the occurrence and composition profiles of 12 frequently used SPAs and three BHT metabolites were investigated in fifty-six sludge samples collected from individual wastewater treatment plants in China. Eleven SPAs were positively found in the sludge samples, in which, to our knowledge, eight SPA compounds were identified for the first time in the environment. BHT, 4-tert-octylphenol (4-tOP), and 2,4,6-tri-tert-bultylphenol (AO 246) were the most dominant SPAs in the sludge at mean concentrations of 4.14 mu g/g, 374 ng/g, and 98.1 ng/g d.w. (dry weight). Meanwhile, three BHT metabolites, including 3,5-di-tert-butyl-4-hydroxybenzaldehyde (BHT-CHO), 2,6-di-tert-butyl-1,4-benzoquinone (BHT-Q), and 2,6-di-tert-butyl-4-hydroxy-4-methyl-2,5-cyclohexadienone (BHT-quinol), were also found in most of the samples (>98.2%) with mean concentrations of 141, 562, and 225 ng/g d.w., respectively. The activated sludge system (anaerobic, anoxic, and oxic tanks) of a wastewater treatment plant was further investigated for the removal efficiencies of the SPAs. High removal efficiencies (80.1-89.2%) were found for the six detected SPAs in the aqueous phase, while generation of large proportions of the three BHT metabolites was also observed. |
| 研究领域[WOS] | Engineering, Environmental ; Environmental Sciences |
| WOS记录号 | WOS:000349806400013 |
| 公开日期 | 2016-03-15 |
| 源URL | [http://ir.rcees.ac.cn/handle/311016/32633]  |
| 专题 | 生态环境研究中心_环境化学与生态毒理学国家重点实验室 |
| 推荐引用方式 GB/T 7714 | Liu, Runzeng,Song, Shanjun,Lin, Yongfeng,et al. Occurrence of Synthetic Phenolic Antioxidants and Major Metabolites in Municipal Sewage Sludge in China[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2015,49(4):2073-2080. |
| APA | Liu, Runzeng,Song, Shanjun,Lin, Yongfeng,Ruan, Ting,&Jiang, Guibin.(2015).Occurrence of Synthetic Phenolic Antioxidants and Major Metabolites in Municipal Sewage Sludge in China.ENVIRONMENTAL SCIENCE & TECHNOLOGY,49(4),2073-2080. |
| MLA | Liu, Runzeng,et al."Occurrence of Synthetic Phenolic Antioxidants and Major Metabolites in Municipal Sewage Sludge in China".ENVIRONMENTAL SCIENCE & TECHNOLOGY 49.4(2015):2073-2080. |
入库方式： OAI收割
来源：生态环境研究中心
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