Enhanced visible-light-driven photocatalytic performance of porous graphitic carbon nitride
文献类型：期刊论文
| 作者 | Chang, F; Li, CL; Luo, JR; Xie, YC; Deng, BQ; Hu, XF
|
| 刊名 | APPLIED SURFACE SCIENCE
 |
| 出版日期 | 2015-12-15 |
| 卷号 | 358页码:270-277 |
| 关键词 | Porousg-C3N4 Nitric acid Photocatalysis Rhodamine B Mechanisma |
| ISSN号 | 0169-4332 |
| 产权排序 | [Chang, Fei; Li, Chenlu; Luo, Jieru; Xie, Yunchao; Deng, Baoqing] Univ Shanghai Sci & Technol, Sch Environm & Architecture, Shanghai 200093, Peoples R China; [Hu, Xuefeng] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Shandong, Peoples R China |
| 通讯作者 | Chang, F (reprint author), Univ Shanghai Sci & Technol, Sch Environm & Architecture, Shanghai 200093, Peoples R China. feichang@usst.edu.cn ; xfhu@yic.ac.cn |
| 英文摘要 | In this study, a series of porous graphitic carbon nitride (g-C3N4) materials were fabricated through a direct pyrolysis of protonated melamine by nitric acid solution. These as-prepared porous samples were characterized by a collection of analytical techniques. It was found that a proper concentration of nitric acid solution involved facilitated to generate samples in tube-like morphology with numerous pores, identified with X-ray diffraction patterns, FT-IR spectra, SEM, TEM, and BET measurements. These g-C3N4 samples were subjected to photocatalytic degradation of dye Rhodamine B (RhB) in aqueous under visible-light irradiation. Under identical conditions, those porous g-C3N4 samples showed significantly improved catalytic performance in comparison with the sample prepared without the introduction of nitric acid. In particularly, the best candidate, sample M1:1, showed an apparent reaction rate nearly 6.2 times that of the unmodified counterpart. The enhancement of photocatalytic performance could be attributed to the favorable porous structure with the enlarged specific surface area and the suitable electronic structure as well. In addition, ESR measurements were conducted for the sake of proposing a photocatalytic degradation mechanism. (C) 2015 Elsevier B.V. All rights reserved. |
| 研究领域[WOS] | Chemistry ; Materials Science ; Physics |
| 关键词[WOS] | TEMPLATE-FREE SYNTHESIS ; HYDROGEN EVOLUTION ; H-2 EVOLUTION ; QUANTUM DOTS ; DOPED G-C3N4 ; IRRADIATION ; DEGRADATION ; WATER ; NANOSHEETS ; SEMICONDUCTOR |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000366220400033 |
| 源URL | [http://ir.yic.ac.cn/handle/133337/9317]  |
| 专题 | 烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室 |
| 推荐引用方式 GB/T 7714 | Chang, F,Li, CL,Luo, JR,et al. Enhanced visible-light-driven photocatalytic performance of porous graphitic carbon nitride[J]. APPLIED SURFACE SCIENCE,2015,358:270-277. |
| APA | Chang, F,Li, CL,Luo, JR,Xie, YC,Deng, BQ,&Hu, XF.(2015).Enhanced visible-light-driven photocatalytic performance of porous graphitic carbon nitride.APPLIED SURFACE SCIENCE,358,270-277. |
| MLA | Chang, F,et al."Enhanced visible-light-driven photocatalytic performance of porous graphitic carbon nitride".APPLIED SURFACE SCIENCE 358(2015):270-277. |
入库方式： OAI收割
来源：烟台海岸带研究所
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