Electron-Acceptor-Dependent Light Absorption, Excited-State Relaxation, and Charge Generation in Triphenylamine Dye-Sensitized Solar Cells
文献类型：期刊论文
| 作者 | Li,Renzhi; Zhang,Min; Yan,Cancan; Yao,Zhaoyang; Zhang,Jing; Wang,Peng |
| 刊名 | chemsuschem
 |
| 出版日期 | 2015 |
| 卷号 | 8期号:1页码:97-104 |
| 关键词 | ORGANIC-DYES HIGH-EFFICIENCY TRANSFER DYNAMICS ENERGY-DISSIPATION SURFACE-STATES X-RAYS FEMTOSECOND TITANIA RECOMBINATION SPECTROSCOPY |
| 通讯作者 | wang,p |
| 英文摘要 | by choosing a simple triphenylamine electron donor, we herein compare the influence of electron acceptors benzothiadiazole benzoic acid (btba) and cyanoacrylic acid (ca), on energy levels, light absorption, and dynamics of excited-state evolution and electron injection. dft and time-dependent dft calculations disclosed remarkable intramolecular conformational changes for the excited states of these two donor-acceptor dyes. photoinduced dihedral angle variation occurs to the tri-phenylamine unit in the ca dye and backbone planarization happens to conjugated aromatic blocks in the btba dye. femtosecond spectroscopic measurements suggested the crucial role of having a long excited-state lifetime in maintaining a high electron-injection yield because a reduced driving force for a low energy-gap dye can result in slower electron-injection dynamics. |
| 收录类别 | SCI |
| 语种 | 英语 |
| 公开日期 | 2016-05-03 |
| 源URL | [http://ir.ciac.jl.cn/handle/322003/64627]  |
| 专题 | 长春应用化学研究所_长春应用化学研究所知识产出_期刊论文 |
| 推荐引用方式 GB/T 7714 | Li,Renzhi,Zhang,Min,Yan,Cancan,et al. Electron-Acceptor-Dependent Light Absorption, Excited-State Relaxation, and Charge Generation in Triphenylamine Dye-Sensitized Solar Cells[J]. chemsuschem,2015,8(1):97-104. |
| APA | Li,Renzhi,Zhang,Min,Yan,Cancan,Yao,Zhaoyang,Zhang,Jing,&Wang,Peng.(2015).Electron-Acceptor-Dependent Light Absorption, Excited-State Relaxation, and Charge Generation in Triphenylamine Dye-Sensitized Solar Cells.chemsuschem,8(1),97-104. |
| MLA | Li,Renzhi,et al."Electron-Acceptor-Dependent Light Absorption, Excited-State Relaxation, and Charge Generation in Triphenylamine Dye-Sensitized Solar Cells".chemsuschem 8.1(2015):97-104. |
入库方式： OAI收割
来源：长春应用化学研究所
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