Levels and speciation of arsenic in the atmosphere in Beijing, China
文献类型：期刊论文
| 作者 | Yang GS(杨国胜); 马玲玲(多); Xu DD(徐殿斗) ; Yang, GS; Ma, LL; Xu, DD; Li, J; He, TT; Liu, LY; Jia, HL
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| 刊名 | CHEMOSPHERE
 |
| 出版日期 | 2012 |
| 卷号 | 87期号:8页码:845-850 |
| 关键词 | Arsenic Speciation Air Beijing Risk assessment |
| 英文摘要 | Arsenic levels and speciation in the total suspended particles (TSPs) were quantitatively determined by high performance liquid chromatography on-line coupled with hydride generation atomic fluorescence spectrometry in Beijing, China from February 2009 to March 2011. The high TSP levels fluctuated between 0.07 and 0.79 mg m(-3), with a mean level of 0.32 +/- 0.17 mg m(-3). The total arsenic concentrations ranged from 0.03 to 0.31 mu g m(-3) (mean: 0.13 +/- 0.06 mu g m(-3)) in Beijing's air. The concentrations of As(III) and As(V) ranged from 0.73 to 20 ng m(-3) (mean: 4.7 +/- 3.6 ng m(-3)) and from 14 to 2.5 x 10(2) ng m(-3) (mean: 67 35 ng m-3), respectively. As levels and speciation demonstrated relative higher levels in spring and autumn and lower values in summer and winter. As(V) accounted for 81-99% of the extractable species in the TSP samples which showed that As(V) was the major fraction of the extractable As. Organoarsenic species, monomethylarsonate (MMA) and dimethylarsinate (DMA) were not found in all samples. Higher values of enrichment factors demonstrated that arsenic in TSP mainly come from anthropogenic sources. High As and its species levels in air and respiratory exposure (0.30-0.84 mu g d(-1)) attributed to higher excess cancer risk ((4.2 +/- 2.0) x 10(-4)) for people in Beijing. (C) 2012 Elsevier Ltd. All rights reserved. |
| 学科主题 | Environmental Sciences & Ecology |
| 收录类别 | SCI |
| WOS记录号 | WOS:000302988100003 |
| 公开日期 | 2016-05-03 |
| 源URL | [http://ir.ihep.ac.cn/handle/311005/224070]  |
| 专题 | 高能物理研究所_院士 高能物理研究所_多学科研究中心 |
| 推荐引用方式 GB/T 7714 | Yang GS,Ma LL,Xu DD,et al. Levels and speciation of arsenic in the atmosphere in Beijing, China[J]. CHEMOSPHERE,2012,87(8):845-850. |
| APA | 杨国胜.,马玲玲.,徐殿斗.,Yang, GS.,Ma, LL.,...&柴之芳.(2012).Levels and speciation of arsenic in the atmosphere in Beijing, China.CHEMOSPHERE,87(8),845-850. |
| MLA | 杨国胜,et al."Levels and speciation of arsenic in the atmosphere in Beijing, China".CHEMOSPHERE 87.8(2012):845-850. |
入库方式： OAI收割
来源：高能物理研究所
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