Modeling of kinetic-based catalyst grading for upgrading shale oil hydrogenation
文献类型：期刊论文
| 作者 | Dai, Fei1,2; Wang, Hongyan1; Gong, Maoming1; Li, Chunshan2; Muhammad, Yaseen2; Li, Zengxi1 |
| 刊名 | FUEL
 |
| 出版日期 | 2016-02-15 |
| 卷号 | 166期号:FEB页码:19-23 |
| 关键词 | Catalyst grading Kinetic model Shale oil hydrogenation Optimization |
| ISSN号 | 0016-2361 |
| 英文摘要 | In this work, shale oil hydrogenation was upgraded in a two fixed-bed reactors to maximize light fraction with ultra-low sulfur and nitrogen. Three types of catalyst grading for shale oil hydroprotection, hydrofining, and hydrocracking were investigated to evaluate the hydrogenation performance. A lumping kinetic model of hydrodesulfurization, hydrodenitrification, and hydrocracking based on catalysts grading was established for the first time. Model parameters were determined using the Levenberg-Marquardt optimization algorithm. Results revealed that the model could accurately predict the removal rations of sulfur, nitrogen, and desired product yields in shale oil hydrogenation under different catalyst grading. Thus, the model can be used for optimization of catalyst stacking to meet the requirements of hydrogenation products. (C) 2015 Elsevier Ltd. All rights reserved. |
| WOS标题词 | Science & Technology ; Technology |
| 类目[WOS] | Energy & Fuels ; Engineering, Chemical |
| 研究领域[WOS] | Energy & Fuels ; Engineering |
| 关键词[WOS] | COAL-TAR ; DISTILLATION FRACTIONS ; HEAVY MAZUTE ; HYDROCRACKING ; TEMPERATURE ; DIESEL ; YIELD |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000365627700003 |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/19894]  |
| 专题 | 过程工程研究所_多相复杂系统国家重点实验室 |
| 作者单位 | 1.Chinese Acad Sci, Grad Univ, Coll Chem & Chem Engn, Beijing 100049, Peoples R China 2.Chinese Acad Sci, State Key Lab Multiphase Complex Syst, Inst Proc Engn, Beijing Key Lab Ion Liquids Clean Proc, Beijing 100190, Peoples R China |
| 推荐引用方式 GB/T 7714 | Dai, Fei,Wang, Hongyan,Gong, Maoming,et al. Modeling of kinetic-based catalyst grading for upgrading shale oil hydrogenation[J]. FUEL,2016,166(FEB):19-23. |
| APA | Dai, Fei,Wang, Hongyan,Gong, Maoming,Li, Chunshan,Muhammad, Yaseen,&Li, Zengxi.(2016).Modeling of kinetic-based catalyst grading for upgrading shale oil hydrogenation.FUEL,166(FEB),19-23. |
| MLA | Dai, Fei,et al."Modeling of kinetic-based catalyst grading for upgrading shale oil hydrogenation".FUEL 166.FEB(2016):19-23. |
入库方式： OAI收割
来源：过程工程研究所
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