Carbon-Number-Based Kinetics, Reactor Modeling, and Process Simulation for Coal Tar Hydrogenation
文献类型：期刊论文
| 作者 | Dai, Fei1,2; Wang, Hongyan1; Gong, Maoming1; Li, Chunshan2; Li, Zengxi1; Zhang, Suojiang2 |
| 刊名 | ENERGY & FUELS
 |
| 出版日期 | 2015-11-01 |
| 卷号 | 29期号:11页码:7532-7541 |
| ISSN号 | 0887-0624 |
| 英文摘要 | A new carbon-number-based kinetic model containing 18 hydrocarbon groups was developed in this work to describe coal tar hydrogenation, and the kinetic parameters were determined by means of fitting the experimental data, obtained in a two-stage fixed-bed reactor hydrogenation experiment, under various operating conditions. Model validation revealed that experimental data considerably agreed with expected outcomes. On this basis, a non-isothermal reactor model based on mass balance and energy balance as well as the proposed reaction kinetic model were constructed to further investigate the behavior of the hydrogenation fixed-bed unit, and the reactor model applied in a bench-scale plant of coal tar hydrogenation accurately simulated and predicted the yield distribution of carbon number products and the temperature profile along with the reactor. In addition, the entire process simulation for coal tar hydrogenation was developed using Aspen Plus. The simulation provided a significant guide for the optimization and design of industrial-scale hydrogenation. |
| WOS标题词 | Science & Technology ; Technology |
| 类目[WOS] | Energy & Fuels ; Engineering, Chemical |
| 研究领域[WOS] | Energy & Fuels ; Engineering |
| 关键词[WOS] | INDUSTRIAL HYDROCRACKING UNIT ; CLEAN LIQUID FUELS ; VACUUM GAS OILS ; MOLECULAR RECONSTRUCTION ; SIMULTANEOUS HYDRODESULFURIZATION ; HYDROTREATING PROCESSES ; STEAM CRACKING ; RESIDUE ; OPTIMIZATION ; FEEDSTOCKS |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000365462400071 |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/19900]  |
| 专题 | 过程工程研究所_多相复杂系统国家重点实验室 |
| 作者单位 | 1.Grad Univ Chinese Acad Sci, Coll Chem & Chem Engn, Beijing 100049, Peoples R China 2.Chinese Acad Sci, Beijing Key Lab Ion Liquids Clean Proc, State Key Lab Multiphase Complex Syst, Inst Proc Engn, Beijing 100190, Peoples R China |
| 推荐引用方式 GB/T 7714 | Dai, Fei,Wang, Hongyan,Gong, Maoming,et al. Carbon-Number-Based Kinetics, Reactor Modeling, and Process Simulation for Coal Tar Hydrogenation[J]. ENERGY & FUELS,2015,29(11):7532-7541. |
| APA | Dai, Fei,Wang, Hongyan,Gong, Maoming,Li, Chunshan,Li, Zengxi,&Zhang, Suojiang.(2015).Carbon-Number-Based Kinetics, Reactor Modeling, and Process Simulation for Coal Tar Hydrogenation.ENERGY & FUELS,29(11),7532-7541. |
| MLA | Dai, Fei,et al."Carbon-Number-Based Kinetics, Reactor Modeling, and Process Simulation for Coal Tar Hydrogenation".ENERGY & FUELS 29.11(2015):7532-7541. |
入库方式： OAI收割
来源：过程工程研究所
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