Aqueous Carbonation of Steel Slag: A Kinetics Study
文献类型：期刊论文
| 作者 | Tu, Maoxia1,2; Zhao, Hongxin1; Lei, Ze2; Wang, Lina1; Chen, Desheng1; Yu, Hongdong1; Qi, Tao1 |
| 刊名 | ISIJ INTERNATIONAL
 |
| 出版日期 | 2015 |
| 卷号 | 55期号:11页码:2509-2514 |
| 关键词 | kinetics aqueous carbonation carbon dioxide sequestration steel slag |
| ISSN号 | 0915-1559 |
| 英文摘要 | In this study, the kinetics of aqueous carbonation of steel slag in an atmospheric three-phase system containing steel slag, water, and CO2 gas was studied. Also, some factors likely affecting this process were investigated, such as reaction time and temperature, steel slag particle size (d(0.5)), CO2 flow rate, and the mass ratio of liquid to solid (L/S). The particle size of steel slag and the reaction temperature were found to be the major factors affecting the carbonation degree. The carbonation degree was determined to be 26.4% under the following conditions: reaction time of 3 h, temperature of 60 degrees C, CO2 flow rate of 600 ml/min, d(0.5) = 12.8 mu m, L/S=10, corresponding to a capacity of 0.264 kg CO2/kg steel slag. The experimental results were employed to study the reaction mechanism using the shrinking core model. The aqueous carbonation process of steel slag was found to be limited by the diffusion of calcium carbonate through the product layer. The apparent activation energy of the aqueous carbonation of steel slag was found to be 4.8 kJ/mol. It was confirmed that aqueous carbonation of steel slag is an effective approach for enhancing the CO2-sequestration capacity and reducing the environmental impacts of steel slag. |
| WOS标题词 | Science & Technology ; Technology |
| 类目[WOS] | Metallurgy & Metallurgical Engineering |
| 研究领域[WOS] | Metallurgy & Metallurgical Engineering |
| 关键词[WOS] | ACCELERATED CARBONATION ; MINERAL SEQUESTRATION ; CO2 SEQUESTRATION ; STEELMAKING SLAG ; PRESSURE |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000365372400031 |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/19892]  |
| 专题 | 过程工程研究所_湿法冶金清洁生产技术国家工程实验室 |
| 作者单位 | 1.Chinese Acad Sci, Inst Proc Engn, Natl Engn Lab Hydromet Cleaner Prod Technol, Key Lab Green Proc & Engn, Beijing 100190, Peoples R China 2.China Univ Min & Technol, Beijing Sch Chem & Environm Engn, Beijing 100083, Peoples R China |
| 推荐引用方式 GB/T 7714 | Tu, Maoxia,Zhao, Hongxin,Lei, Ze,et al. Aqueous Carbonation of Steel Slag: A Kinetics Study[J]. ISIJ INTERNATIONAL,2015,55(11):2509-2514. |
| APA | Tu, Maoxia.,Zhao, Hongxin.,Lei, Ze.,Wang, Lina.,Chen, Desheng.,...&Qi, Tao.(2015).Aqueous Carbonation of Steel Slag: A Kinetics Study.ISIJ INTERNATIONAL,55(11),2509-2514. |
| MLA | Tu, Maoxia,et al."Aqueous Carbonation of Steel Slag: A Kinetics Study".ISIJ INTERNATIONAL 55.11(2015):2509-2514. |
入库方式： OAI收割
来源：过程工程研究所
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