Anti-sintering ZrO2-modified Ni/alpha-Al2O3 catalyst for CO methanation
文献类型：期刊论文
| 作者 | Liu, Qing1; Gu, Fangna1; Zhong, Ziyi2; Xu, Guangwen1; Su, Fabing1 |
| 刊名 | RSC ADVANCES
 |
| 出版日期 | 2016 |
| 卷号 | 6期号:25页码:20979-20986 |
| 关键词 | SYNTHETIC NATURAL-GAS NI-BASED CATALYSTS NI/AL2O3 CATALYSTS CARBON-DIOXIDE HYDROGENOLYSIS PERFORMANCE PROGRESS LIGNIN WATER |
| ISSN号 | 2046-2069 |
| 通讯作者 | Gu, FN |
| 英文摘要 | To obviously reduce the sintering behavior of Ni particles in Ni/alpha-Al2O3 catalysts during CO methanation reaction, ZrO2 was deposited onto the Ni/a-Al2O3 catalyst surface by a modified impregnation method. It was observed that the ZrO2-modified catalyst with an appropriate amount of ZrO2 showed enhanced catalytic activity due to the increased H-2 uptake and Ni dispersion. During the 103h-lifetime test, the ZrO2-modified catalyst exhibited higher stability and anti-sintering performance than the unmodified one, because the partial coverage of ZrO2 particles could effectively prevent Ni particles from sintering during the reaction at high temperatures. The findings obtained in this study should be conducive to the design and development of supported metal catalysts for high temperature reactions with enhanced stability. |
| WOS标题词 | Science & Technology ; Physical Sciences |
| 学科主题 | Chemistry, Multidisciplinary ; Chemistry |
| 类目[WOS] | Chemistry, Multidisciplinary |
| 研究领域[WOS] | Chemistry |
| 关键词[WOS] | SYNTHETIC NATURAL-GAS ; NI-BASED CATALYSTS ; NI/AL2O3 CATALYSTS ; CARBON-DIOXIDE ; HYDROGENOLYSIS ; PERFORMANCE ; PROGRESS ; LIGNIN ; WATER |
| 收录类别 | SCI |
| 原文出处 | ROYAL SOC CHEMISTRY |
| 语种 | 英语 |
| WOS记录号 | WOS:000371019000063 |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/20707]  |
| 专题 | 过程工程研究所_研究所（批量导入） |
| 作者单位 | 1.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China 2.ASTAR, Inst Chem Engn & Sci, 1 Pesek Rd, Singapore 627833, Singapore |
| 推荐引用方式 GB/T 7714 | Liu, Qing,Gu, Fangna,Zhong, Ziyi,et al. Anti-sintering ZrO2-modified Ni/alpha-Al2O3 catalyst for CO methanation[J]. RSC ADVANCES,2016,6(25):20979-20986. |
| APA | Liu, Qing,Gu, Fangna,Zhong, Ziyi,Xu, Guangwen,&Su, Fabing.(2016).Anti-sintering ZrO2-modified Ni/alpha-Al2O3 catalyst for CO methanation.RSC ADVANCES,6(25),20979-20986. |
| MLA | Liu, Qing,et al."Anti-sintering ZrO2-modified Ni/alpha-Al2O3 catalyst for CO methanation".RSC ADVANCES 6.25(2016):20979-20986. |
入库方式： OAI收割
来源：过程工程研究所
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