Alignment-Dependent Fluorescence Emission Induced by Tunnel Ionization of Carbon Dioxide from Lower-Lying Orbitals
文献类型：期刊论文
| 作者 | Yao, Jinping1; Li, Guihua1,7; Jia, Xinyan2; Hao, Xiaolei3,4; Zeng, Bin1; Jing, Chenrui1,7; Chu, Wei1; Ni, Jielei1,7; Zhang, Haisu1,7; Xie, Hongqiang1,7 |
| 刊名 | PHYSICAL REVIEW LETTERS
 |
| 出版日期 | 2013-09-26 |
| 卷号 | 111期号:13 |
| 英文摘要 | The study of the ionization process of molecules in an intense infrared laser field is of paramount interest in strong-field physics and constitutes the foundation of imaging of molecular valence orbitals and attosecond science. We show measurement of alignment-dependent ionization probabilities of the lower-lying orbitals of the molecules by experimentally detecting the alignment dependence of fluorescence emission from tunnel ionized carbon dioxide molecules. The experimental measurements are compared with the theoretical calculations of the strong field approximation and molecular Ammosov-Delone-Krainov models. Our results demonstrate the feasibility of an all-optical approach for probing the ionization dynamics of lower-lying orbitals of molecules, which is until now still difficult to achieve by other techniques. Moreover, the deviation between the experimental and theoretical results indicates the incompleteness of current theoretical models for describing strong field ionization of molecules. |
| WOS标题词 | Science & Technology ; Physical Sciences |
| 类目[WOS] | Physics, Multidisciplinary |
| 研究领域[WOS] | Physics |
| 关键词[WOS] | HARMONIC-GENERATION ; MULTIPLE ORBITALS ; LASER FIELDS ; MOLECULES ; DYNAMICS |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000325364300009 |
| 公开日期 | 2016-05-09 |
| 源URL | [http://ir.wipm.ac.cn/handle/112942/915]  |
| 专题 | 武汉物理与数学研究所_原子分子光物理研究部 |
| 作者单位 | 1.Chinese Acad Sci, Shanghai Inst Opt & Fine Mech, State Key Lab High Field Laser Phys, Shanghai 201800, Peoples R China 2.Southwest Jiaotong Univ, Quantum Optoelect Lab, Chengdu 610031, Peoples R China 3.Peking Univ, Ctr Appl Phys & Technol, Key Lab High Energy Dens Phys Simulat, Beijing 100084, Peoples R China 4.Inst Appl Phys & Computat Math, Beijing 100088, Peoples R China 5.Natl Univ Def Technol, Dept Phys, Changsha 410073, Hunan, Peoples R China 6.Chinese Acad Sci, Wuhan Inst Phys & Math, State Key Lab Magnet Resonance & Atom & Mol Phys, Wuhan 430071, Peoples R China 7.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Yao, Jinping,Li, Guihua,Jia, Xinyan,et al. Alignment-Dependent Fluorescence Emission Induced by Tunnel Ionization of Carbon Dioxide from Lower-Lying Orbitals[J]. PHYSICAL REVIEW LETTERS,2013,111(13). |
| APA | Yao, Jinping.,Li, Guihua.,Jia, Xinyan.,Hao, Xiaolei.,Zeng, Bin.,...&Xu, Zhizhan.(2013).Alignment-Dependent Fluorescence Emission Induced by Tunnel Ionization of Carbon Dioxide from Lower-Lying Orbitals.PHYSICAL REVIEW LETTERS,111(13). |
| MLA | Yao, Jinping,et al."Alignment-Dependent Fluorescence Emission Induced by Tunnel Ionization of Carbon Dioxide from Lower-Lying Orbitals".PHYSICAL REVIEW LETTERS 111.13(2013). |
入库方式： OAI收割
来源：武汉物理与数学研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。