Cavity-Enhanced Field-Free Molecular Alignment at a High Repetition Rate
文献类型：期刊论文
| 作者 | Benko, Craig1; Hua, Linqiang1,2; Allison, Thomas K.3,4; Labaye, Francois1; Ye, Jun1 |
| 刊名 | PHYSICAL REVIEW LETTERS
 |
| 出版日期 | 2015-04-14 |
| 卷号 | 114期号:15 |
| 英文摘要 | Extreme ultraviolet frequency combs are a versatile tool with applications including precision measurement, strong-field physics, and solid-state physics. Here we report on an application of extreme ultraviolet frequency combs and their driving lasers for studying strong-field effects in molecular systems. We perform field-free molecular alignment and high-order harmonic generation with aligned molecules in a gas jet at a repetition rate of 154 MHz using a high-powered optical frequency comb inside a femtosecond enhancement cavity. The cavity-enhanced system provides a means to reach suitable intensities to study field-free molecular alignment and enhance the observable effects of the molecule-field interaction. We observe modulations of the driving field, arising from the nature of impulsive stimulated Raman scattering responsible for coherent molecular rotations. We foresee the impact of this work on the study of molecule-based strong-field physics, with improved precision and a more fundamental understanding of the interaction effects on both the field and molecules. |
| WOS标题词 | Science & Technology ; Physical Sciences |
| 类目[WOS] | Physics, Multidisciplinary |
| 研究领域[WOS] | Physics |
| 关键词[WOS] | RAMAN SELF-CONVERSION ; EXTREME-ULTRAVIOLET ; FREQUENCY COMBS ; LASER-PULSES ; RADIATION ; SPECTROSCOPY ; GENERATION ; EXCITATION |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000352788100003 |
| 公开日期 | 2016-05-09 |
| 源URL | [http://ir.wipm.ac.cn/handle/112942/1070]  |
| 专题 | 武汉物理与数学研究所_原子分子光物理研究部 |
| 作者单位 | 1.Univ Colorado, NIST, JILA, Boulder, CO 80309 USA 2.Chinese Acad Sci, Wuhan Inst Phys & Math, State Key Lab Magnet Resonance & Atom & Mol Phys, Wuhan 430071, Peoples R China 3.SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA 4.SUNY Stony Brook, Dept Phys, Stony Brook, NY 11794 USA |
| 推荐引用方式 GB/T 7714 | Benko, Craig,Hua, Linqiang,Allison, Thomas K.,et al. Cavity-Enhanced Field-Free Molecular Alignment at a High Repetition Rate[J]. PHYSICAL REVIEW LETTERS,2015,114(15). |
| APA | Benko, Craig,Hua, Linqiang,Allison, Thomas K.,Labaye, Francois,&Ye, Jun.(2015).Cavity-Enhanced Field-Free Molecular Alignment at a High Repetition Rate.PHYSICAL REVIEW LETTERS,114(15). |
| MLA | Benko, Craig,et al."Cavity-Enhanced Field-Free Molecular Alignment at a High Repetition Rate".PHYSICAL REVIEW LETTERS 114.15(2015). |
入库方式： OAI收割
来源：武汉物理与数学研究所
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