One-pot catalytic conversion of cellulose to ethylene glycol and other chemicals: From fundamental discovery to potential commercialization
文献类型：期刊论文
| 作者 | Zheng, Mingyuan; Pang, Jifeng; Wang, Aiqin; Zhang, Tao |
| 刊名 | chinese journal of catalysis
 |
| 出版日期 | 2014-05-01 |
| 卷号 | 35期号:5页码:602-613 |
| 关键词 | Biomass Cellulose Ethylene glycol Tungstenic catalyst Hydrogenation |
| 通讯作者 | 张涛 |
| 英文摘要 | the one-pot catalytic conversion of cellulose to ethylene glycol (ceg) is a highly attractive way for biomass utilization to lessen the consumption of fossil energy resources. in this paper, we reviewed the disclosure of the ceg process and the rapid progress in the development of highly efficient and robust catalysts for it. based on our study of tungstenic catalysts, we discuss the reaction mechanism, in which the reaction routes, catalyst states, and catalytic roles of the tungsten species and hydrogenation sites in the cascade reactions are understood clearly. with future applications in mind, the conversion of raw cellulosic biomass and the strategy to develop an efficient ceg process for commercialization are discussed, and a model where the ceg process is incorporated into a bio-refinery process of acetone-n-butanol-ethanol (abe) production is presented. (c) 2014, dalian institute of chemical physics, chinese academy of sciences. published by elsevier b.v. all rights reserved. |
| 学科主题 | 物理化学 |
| WOS标题词 | science & technology ; physical sciences ; technology |
| 类目[WOS] | chemistry, applied ; chemistry, physical ; engineering, chemical |
| 研究领域[WOS] | chemistry ; engineering |
| 关键词[WOS] | tungsten carbide catalysts ; hydrazine decomposition ; lignocellulosic biomass ; selective conversion ; bimetallic catalysts ; raney ni ; microcrystalline cellulose ; 1,2-propylene glycol ; gamma-valerolactone ; ruthenium catalyst |
| 收录类别 | SCI ; ISTP |
| 语种 | 英语 |
| WOS记录号 | WOS:000335622300002 |
| 公开日期 | 2016-05-09 |
| 源URL | [http://cas-ir.dicp.ac.cn/handle/321008/144217]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 作者单位 | Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Liaoning, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zheng, Mingyuan,Pang, Jifeng,Wang, Aiqin,et al. One-pot catalytic conversion of cellulose to ethylene glycol and other chemicals: From fundamental discovery to potential commercialization[J]. chinese journal of catalysis,2014,35(5):602-613. |
| APA | Zheng, Mingyuan,Pang, Jifeng,Wang, Aiqin,&Zhang, Tao.(2014).One-pot catalytic conversion of cellulose to ethylene glycol and other chemicals: From fundamental discovery to potential commercialization.chinese journal of catalysis,35(5),602-613. |
| MLA | Zheng, Mingyuan,et al."One-pot catalytic conversion of cellulose to ethylene glycol and other chemicals: From fundamental discovery to potential commercialization".chinese journal of catalysis 35.5(2014):602-613. |
入库方式： OAI收割
来源：大连化学物理研究所
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