Pathway of H+ in fragmentation of H-2 in 810 nm intense femtosecond laser fields
文献类型:期刊论文
作者 | Guo, Wei1; Lu, Xingqiang2; Zhao, Dan3; Wang, Xinlin1 |
刊名 | physica scripta
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出版日期 | 2014-02-01 |
卷号 | 89期号:2 |
关键词 | bond softening above-threshold dissociation Coulomb explosion light-dressed states |
英文摘要 | we experimentally measured the kinetic energy and angular distributions of fragment ion h+ of h-2 as a function of 810 nm femtosecond laser intensity by using velocity map imaging technique. the reaction pathways of dissociation channels h-2(+) -> h+ + h and h-2(2+) -> h+ + h+ are proposed. the analysis of the angular distribution indicates the net two-photon pathway via the 3 omega crossing dominates over the direct one-photon pathway in channel h-2(+) -> h+ + h. the ionization of h-2(+) to h-2(2+) may be initiated by bond softening and above-threshold dissociation. the relative yield of fragment peaks indicates that dissociation and ionization of h-2(+) are competitive. the lower laser intensities emphasize the dissociation probability of h-2(+), and the higher laser intensities favor higher ionization stages. |
WOS标题词 | science & technology ; physical sciences |
类目[WOS] | physics, multidisciplinary |
研究领域[WOS] | physics |
关键词[WOS] | coulomb explosion ; induced alignment ; molecules ; dynamics ; dissociation ; ionization ; ions |
收录类别 | SCI |
语种 | 英语 |
WOS记录号 | WOS:000331209200005 |
公开日期 | 2016-05-09 |
源URL | [http://cas-ir.dicp.ac.cn/handle/321008/145581] ![]() |
专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
作者单位 | 1.Univ South China, Sch Elect Engn, Hengyang 421001, Peoples R China 2.Univ South China, Sch Nucl Sci & Technol, Hengyang 421001, Peoples R China 3.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China |
推荐引用方式 GB/T 7714 | Guo, Wei,Lu, Xingqiang,Zhao, Dan,et al. Pathway of H+ in fragmentation of H-2 in 810 nm intense femtosecond laser fields[J]. physica scripta,2014,89(2). |
APA | Guo, Wei,Lu, Xingqiang,Zhao, Dan,&Wang, Xinlin.(2014).Pathway of H+ in fragmentation of H-2 in 810 nm intense femtosecond laser fields.physica scripta,89(2). |
MLA | Guo, Wei,et al."Pathway of H+ in fragmentation of H-2 in 810 nm intense femtosecond laser fields".physica scripta 89.2(2014). |
入库方式: OAI收割
来源:大连化学物理研究所
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