Characteristics of Coke Deposition Over a SAPO-34 Catalyst in the Methanol-to-Olefins Reaction
文献类型:期刊论文
作者 | Ying, L.1; Ye, M.2; Cheng, Y. W.1; Li, X.1 |
刊名 | petroleum science and technology
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出版日期 | 2015 |
卷号 | 33期号:9页码:984-991 |
关键词 | MTO SAPO-34 deactivation coke species active center |
英文摘要 | the deactivation of sapo-34 catalyst in the methanol-to-olefins process has been studied at temperatures of 400 to 475 degrees c. the catalyst activity keeps stable before a rapid deactivation occurs at a critical coke content. the analysis of retained coke species showed that methylbenzenes were the most abundant species at lower temperatures (400 degrees c and 425 degrees c), while polycyclic aromatics became the dominant species at 475 degrees c. the growth in the retained coke species with increasing temperature comes from the enhanced reactivity of methylbenzenes and methylnaphthalenes at high reaction temperature, where methylnaphthalenes may function as another active reaction centers. |
WOS标题词 | science & technology ; technology |
类目[WOS] | energy & fuels ; engineering, chemical ; engineering, petroleum |
研究领域[WOS] | energy & fuels ; engineering |
关键词[WOS] | reaction centers ; conversion ; h-sapo-34 ; hsapo-34 |
收录类别 | SCI |
语种 | 英语 |
WOS记录号 | WOS:000357696800004 |
公开日期 | 2016-05-09 |
源URL | [http://cas-ir.dicp.ac.cn/handle/321008/146382] ![]() |
专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
作者单位 | 1.Zhejiang Univ, Dept Chem & Biochem Engn, Hangzhou 310027, Zhejiang, Peoples R China 2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian, Liaoning, Peoples R China |
推荐引用方式 GB/T 7714 | Ying, L.,Ye, M.,Cheng, Y. W.,et al. Characteristics of Coke Deposition Over a SAPO-34 Catalyst in the Methanol-to-Olefins Reaction[J]. petroleum science and technology,2015,33(9):984-991. |
APA | Ying, L.,Ye, M.,Cheng, Y. W.,&Li, X..(2015).Characteristics of Coke Deposition Over a SAPO-34 Catalyst in the Methanol-to-Olefins Reaction.petroleum science and technology,33(9),984-991. |
MLA | Ying, L.,et al."Characteristics of Coke Deposition Over a SAPO-34 Catalyst in the Methanol-to-Olefins Reaction".petroleum science and technology 33.9(2015):984-991. |
入库方式: OAI收割
来源:大连化学物理研究所
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