Direct Imaging Single Methanol Molecule Photocatalysis on Titania
文献类型：期刊论文
| 作者 | Wei, Dong1; Jin, Xianchi1; Huang, Chuanqi2; Dai, Dongxu1; Ma, Zhibo1; Li, Wei-Xue2; Yang, Xueming1 |
| 刊名 | journal of physical chemistry c
 |
| 出版日期 | 2015-08-06 |
| 卷号 | 119期号:31页码:17748-17754 |
| 英文摘要 | photocatalysis of a single methanol molecule on the tio2(110) surface was investigated using a high-resolution scanning tunneling microscopy (stm) technique. three different types of elementary methanol photocatalytic processes, methanol photodissociation, photoinduced migration of formaldehyde, and formaldehyde photodesorption, were clearly observed. detailed chemical structures of the intermediates were obtained through careful comparisons between experimental stm images and theoretical simulations based on density functional theory (dft) calculations. this work demonstrates that elementary photocatalytic processes of a single methanol molecule on the surface can be followed step by step using advanced stm imaging techniques. such a study can provide unprecedented insights into the surface photocatalytic processes and will greatly help us to understand photocatalysis at the most fundamental level. |
| WOS标题词 | science & technology ; physical sciences ; technology |
| 类目[WOS] | chemistry, physical ; nanoscience & nanotechnology ; materials science, multidisciplinary |
| 研究领域[WOS] | chemistry ; science & technology - other topics ; materials science |
| 关键词[WOS] | scanning-tunneling-microscopy ; total-energy calculations ; augmented-wave method ; tio2 photocatalysis ; hydrogen-production ; methyl formate ; x-1 surface ; basis-set ; tio2(110) ; water |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000359332200029 |
| 公开日期 | 2016-05-09 |
| 源URL | [http://cas-ir.dicp.ac.cn/handle/321008/146456]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 作者单位 | 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Liaoning, Peoples R China 2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Liaoning, Peoples R China |
| 推荐引用方式 GB/T 7714 | Wei, Dong,Jin, Xianchi,Huang, Chuanqi,et al. Direct Imaging Single Methanol Molecule Photocatalysis on Titania[J]. journal of physical chemistry c,2015,119(31):17748-17754. |
| APA | Wei, Dong.,Jin, Xianchi.,Huang, Chuanqi.,Dai, Dongxu.,Ma, Zhibo.,...&Yang, Xueming.(2015).Direct Imaging Single Methanol Molecule Photocatalysis on Titania.journal of physical chemistry c,119(31),17748-17754. |
| MLA | Wei, Dong,et al."Direct Imaging Single Methanol Molecule Photocatalysis on Titania".journal of physical chemistry c 119.31(2015):17748-17754. |
入库方式： OAI收割
来源：大连化学物理研究所
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