Communication: Tracking molecular structure deformation and relaxation in real time
文献类型：期刊论文
| 作者 | Wang, Y.1; Liu, W. L.1; Song, Y. F.1; Liu, Y. Q.1; Duo, L. P.2; Jiang, L. L.1; Yu, G. Y.1,3; Yang, Y. Q.1,3 |
| 刊名 | journal of chemical physics
 |
| 出版日期 | 2015-08-07 |
| 卷号 | 143期号:5 |
| 英文摘要 | the ch3i structural deformation induced by strong laser fields is revealed by time-and frequency-resolved ro-vibrational spectra. the experimental results show that the ch3i molecule undergoes ultrafast structural deformation of ch3 "umbrella-closing" induced by the strong fs laser field (more than 10(11)w/cm(2)) and followed by a structural relaxation of "umbrella-opening" within an exponential decay time scale of similar to 620 fs. this study provides a first glimpse of the immense potential of the time- and frequency-resolved vibrational spectra in studying molecular deformation dynamics. (c) 2015 aip publishing llc. |
| WOS标题词 | science & technology ; physical sciences |
| 类目[WOS] | physics, atomic, molecular & chemical |
| 研究领域[WOS] | physics |
| 关键词[WOS] | intense laser fields ; coulomb explosion ; raman-scattering ; dynamics ; spectroscopy ; alignment ; n-2 |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000359377200001 |
| 公开日期 | 2016-05-09 |
| 源URL | [http://cas-ir.dicp.ac.cn/handle/321008/146460]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 作者单位 | 1.Harbin Inst Technol, Dept Phys, Harbin 150001, Peoples R China 2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China 3.China Acad Engn Phys, Inst Fluid Phys, Natl Key Lab Shock Wave & Detonat Phys, Mianyang 621900, Sichuan, Peoples R China |
| 推荐引用方式 GB/T 7714 | Wang, Y.,Liu, W. L.,Song, Y. F.,et al. Communication: Tracking molecular structure deformation and relaxation in real time[J]. journal of chemical physics,2015,143(5). |
| APA | Wang, Y..,Liu, W. L..,Song, Y. F..,Liu, Y. Q..,Duo, L. P..,...&Yang, Y. Q..(2015).Communication: Tracking molecular structure deformation and relaxation in real time.journal of chemical physics,143(5). |
| MLA | Wang, Y.,et al."Communication: Tracking molecular structure deformation and relaxation in real time".journal of chemical physics 143.5(2015). |
入库方式： OAI收割
来源：大连化学物理研究所
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