Enhanced visible-light-driven photocatalytic performance of mesoporous W-Ti-SBA-15 prepared through a facile hydrothermal route
文献类型：期刊论文
| 作者 | Chang, F; Wang, J; Luo, JR; Sun, JR; Deng, BQ; Hu, XF
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| 刊名 | COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS
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| 出版日期 | 2016-06-20 |
| 卷号 | 499页码:69-78 |
| ISSN号 | 0927-7757 |
| 关键词 | W-Ti-SBA15 Visible-light driven Photocatalytic Rhodamine B 2,4-Dichlorophenol Mechanism |
| 通讯作者 | Chang, F (reprint author), Univ Shanghai Sci & Technol, Sch Environm & Architecture, Shanghai 200093, Peoples R China. ; Hu, XF (reprint author), Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Zone Environm Proc & Ecol Remedia, Yantai 264003, Shandong, Peoples R China. feichang@usst.edu.cn ; xfhu@yic.ac.cn |
| 产权排序 | [Chang, Fei; Wang, Jie; Luo, Jieru; Sun, Junrong; Deng, Baoqing] Univ Shanghai Sci & Technol, Sch Environm & Architecture, Shanghai 200093, Peoples R China; [Hu, Xuefeng] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Zone Environm Proc & Ecol Remedia, Yantai 264003, Shandong, Peoples R China |
| 英文摘要 | A facile and one-step hydrothermal procedure was adopted to fabricate a series of W-Ti-SBA15 composites (WTS). These as-prepared composites were systematically characterized by a collection of analytic and spectroscopic techniques. It was found that dual phases of titanium and tungsten species coexisted in mesoporous structures of p6 mm hexagonal symmetry. In addition, these composites were visible-light responsive and exhibited enhanced photocatalytic capability toward degradation of Rhodamine B (RhB) and 2,4-dichlorophenol (2,4-DCP) upon visible-light irradiation in comparison to samples containing single component of titanium or tungsten species. Specifically, the best candidate, sample 8%WTS0.7, had the largest apparent reaction rate constant that was nearly 1.2, 2.1, 2.2, and 5.7 times as high as those of 8%WS, TS0.7, WO3/TiO2, and N-TiO2, respectively. The enhancement of photocatalytic performance was mainly attributed to the well-matched band structures of both components and strengthened visible light adsorption ability, originating from the combination of titania with highly acidic WO3 in SBA15 matrix with large specific surface areas. Active radical species were detected by trapping experiments and a possible photocatalytic mechanism was thus proposed. (C) 2016 Elsevier B.V. All rights reserved. |
| 研究领域[WOS] | Chemistry |
| 关键词[WOS] | SUBSTITUTED SBA-15 ; MOLECULAR-SIEVES ; SOLAR LIGHT ; EFFICIENT ; SILICA ; DEGRADATION ; WO3 ; NANOPARTICLES ; CATALYSTS ; TITANIA |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000375859800009 |
| 源URL | [http://ir.yic.ac.cn/handle/133337/17068]  |
| 专题 | 烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室 |
| 作者单位 | 1.Univ Shanghai Sci & Technol, Sch Environm & Architecture 2.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Zone Environm Proc & Ecol Remedia |
| 推荐引用方式 GB/T 7714 | Chang, F,Wang, J,Luo, JR,et al. Enhanced visible-light-driven photocatalytic performance of mesoporous W-Ti-SBA-15 prepared through a facile hydrothermal route[J]. COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS,2016,499:69-78. |
| APA | Chang, F,Wang, J,Luo, JR,Sun, JR,Deng, BQ,&Hu, XF.(2016).Enhanced visible-light-driven photocatalytic performance of mesoporous W-Ti-SBA-15 prepared through a facile hydrothermal route.COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS,499,69-78. |
| MLA | Chang, F,et al."Enhanced visible-light-driven photocatalytic performance of mesoporous W-Ti-SBA-15 prepared through a facile hydrothermal route".COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS 499(2016):69-78. |
入库方式： OAI收割
来源：烟台海岸带研究所
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