Synthesis of Thin-Layered Molybdenum Disulfide-Based Polyaniline Nanointerfaces for Enhanced Direct Electrochemical DNA Detection
文献类型：期刊论文
| 作者 | Yang, Tao1; Meng, Le1; Chen, Huaiyin1; Luo, Shizhong1; Li, Weihua2,3; Jiao, Kui1 |
| 刊名 | ADVANCED MATERIALS INTERFACES
 |
| 出版日期 | 2016-04-08 |
| 卷号 | 3期号:7 |
| 英文摘要 | The low electronic conductivity limits the application of molybdenum disulfide (MoS2) in electrochemical sensing field, let alone the label-free and self-signal amplification DNA sensing. Aiming at this problem, a novel polyaniline-molybdenum disulfide (PANI-MoS2) nanocomposite through a facile oxidation polymerization aniline monomer on the thin-layer MoS2 matrix is prepared, which is preobtained via a simple ultrasonic exfoliation method. It is generally appreciated that conducting polymers, e.g., polyaniline (PANI), can work as a direct transducer based on themselves-signal without any label or indicator. Moreover, MoS2 not only serves as an excellent conductive skeleton provided a high electrolytic accessible surface area for redox-active PANI, but also supports a direct path for electron transfer. Therefore, the hybrid of PANI and MoS2 exhibits superior electrochemical performance to pure PANI and MoS2, and can be considered as a superior candidate for direct and label-free electrochemical DNA sensing. A series of experiments are performed to investigate the effect of synthetic conditions (component, dosage of MoS2, and reaction time) on probe DNA (pDNA) immobilization and hybridization adopting the PANI self-signal as the measure signal. The results show that the dosage of MoS2 has a more influence on pDNA immobilization and hybridization. |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000374153000009 |
| 版本 | 出版稿 |
| 源URL | [http://ir.qdio.ac.cn/handle/337002/131012]  |
| 专题 | 海洋研究所_海洋腐蚀与防护研究发展中心 |
| 作者单位 | 1.Qingdao Univ Sci & Technol, Coll Chem & Mol Engn, Key Lab Sensor Anal Tumor Marker, Shandong Prov Key Lab Biochem Anal,Educ Minist, Qingdao 266042, Peoples R China 2.Chinese Acad Sci, Inst Oceanol, Qingdao 266071, Peoples R China 3.Qingdao Technol Univ, Cooperat Innovat Ctr Engn Construct & Safety Shan, Qingdao 266033, Peoples R China |
| 推荐引用方式 GB/T 7714 | Yang, Tao,Meng, Le,Chen, Huaiyin,et al. Synthesis of Thin-Layered Molybdenum Disulfide-Based Polyaniline Nanointerfaces for Enhanced Direct Electrochemical DNA Detection[J]. ADVANCED MATERIALS INTERFACES,2016,3(7). |
| APA | Yang, Tao,Meng, Le,Chen, Huaiyin,Luo, Shizhong,Li, Weihua,&Jiao, Kui.(2016).Synthesis of Thin-Layered Molybdenum Disulfide-Based Polyaniline Nanointerfaces for Enhanced Direct Electrochemical DNA Detection.ADVANCED MATERIALS INTERFACES,3(7). |
| MLA | Yang, Tao,et al."Synthesis of Thin-Layered Molybdenum Disulfide-Based Polyaniline Nanointerfaces for Enhanced Direct Electrochemical DNA Detection".ADVANCED MATERIALS INTERFACES 3.7(2016). |
入库方式： OAI收割
来源：海洋研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。