Production of cyclohexane from lignin degradation compounds over Ni/ZrO2-SiO2 catalysts
文献类型：期刊论文
| 作者 | Zhang, Xinghua1,2; Wang, Tiejun1; Ma, Longlong1; Zhang, Qi1; Huang, Xiaoming1,2; Yu, Yuxiao1,2 |
| 刊名 | applied energy
 |
| 出版日期 | 2013-12-01 |
| 卷号 | 112页码:533-538 |
| 关键词 | Lignin Phenolic compounds Ni/ZrO2-SiO2 Cyclohexane Hydrodeoxygenation (HDO) |
| 英文摘要 | the main products of lignin degradation are phenolic compounds. it is meaningful to study the processes by which cyclohexane is produced from phenolic compounds via hydrodeoxygenation (hdo), because it could be used as fuel additives, chemical feedstock and solvent. in this work, support material zro2-sio2 mixed oxides with different si/zr ratio were synthesized, and a series of ni/sio2-zro2 catalysts with different ni loading were prepared by impregnation method. the exploration of hdo process was carried out using phenol and guaiacol as model compounds. effects of si/zr ratio, ni loading and reaction temperature on conversion of phenol and guaiacol as well as distribution of hdo products were systematically investigated. the results showed that almost all of phenol and guaiacol could be effectively converted into o-free products. and the selectivity of cyclohexane was in excess of 90%. (c) 2013 elsevier ltd. all rights reserved. |
| WOS标题词 | science & technology ; technology |
| 类目[WOS] | energy & fuels ; engineering, chemical |
| 研究领域[WOS] | energy & fuels ; engineering |
| 关键词[WOS] | ethanol-production ; hydrodeoxygenation ; conversion ; acid |
| 收录类别 | SCI ; ISTP |
| 语种 | 英语 |
| WOS记录号 | WOS:000329377800056 |
| 源URL | [http://ir.giec.ac.cn/handle/344007/10035]  |
| 专题 | 中国科学院广州能源研究所 |
| 作者单位 | 1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy & Gas Hydrate, Guangzhou 510640, Peoples R China 2.Chinese Acad Sci, Grad Sch, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhang, Xinghua,Wang, Tiejun,Ma, Longlong,et al. Production of cyclohexane from lignin degradation compounds over Ni/ZrO2-SiO2 catalysts[J]. applied energy,2013,112:533-538. |
| APA | Zhang, Xinghua,Wang, Tiejun,Ma, Longlong,Zhang, Qi,Huang, Xiaoming,&Yu, Yuxiao.(2013).Production of cyclohexane from lignin degradation compounds over Ni/ZrO2-SiO2 catalysts.applied energy,112,533-538. |
| MLA | Zhang, Xinghua,et al."Production of cyclohexane from lignin degradation compounds over Ni/ZrO2-SiO2 catalysts".applied energy 112(2013):533-538. |
入库方式： OAI收割
来源：广州能源研究所
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