Synthesis Gas from Pyrolysis of Cedar Sawdust as Biomass Materials: Characterization and Catalytic Performance of Nickel-Based Monolithic Catalyst
文献类型：期刊论文
| 作者 | Lu Min1,2; Lue Pengmei1; Yuan Zhenhong1; Li Huiwen1; Xu Jingliang1 |
| 刊名 | chinese journal of catalysis
 |
| 出版日期 | 2011-06-01 |
| 卷号 | 32期号:6页码:1017-1021 |
| 关键词 | biomass synthesis gas cordierite acid treatment nickel oxide tar conversion carbon deposition |
| 英文摘要 | a series of monolithic catalysts with different nio loadings were prepared by supported on the acid treated cordierite. their specific surface area, pore volume, pore distribution, and catalytic performance in the reforming reaction of biomass pyrolysis gas for synthesis gas were studied. the results show that the specific surface area and pore volume of the cordierite after acid treatment are up to 156 m(2)/g and 0.099 m(3)/g respectively. however, with increasing nickel oxide loading, the specific surface area and pore volume of the catalyst decrease greatly and then tend to steady. the effect of nickel oxide loading on gas composition is quite small, and the total content of h(2) and co is maintained at 90%. the tar conversion is not affected by the specific surface area of the catalysts. after 6 h catalytic reaction, the structure of the catalysts with 28% nio does not change, and the quantity of carbon deposition is about 1%. the tar conversion decreases from 87.4% to 81.3%. it is suggested that the nickel-based catalyst has relatively stable activity under high tar concentration conditions, which is attributed to the high dispersion of nickel particles on the support and high stability of the catalyst phase structure. |
| WOS标题词 | science & technology ; physical sciences ; technology |
| 类目[WOS] | chemistry, applied ; chemistry, physical ; engineering, chemical |
| 研究领域[WOS] | chemistry ; engineering |
| 关键词[WOS] | fischer-tropsch synthesis ; fluidized-bed ; tar elimination ; gasification ; steam ; reduction ; olivine ; syngas ; nox |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000292429000018 |
| 源URL | [http://ir.giec.ac.cn/handle/344007/10361]  |
| 专题 | 中国科学院广州能源研究所 |
| 作者单位 | 1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy & Gas Hydrate, Guangzhou 510640, Guangdong, Peoples R China 2.Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Lu Min,Lue Pengmei,Yuan Zhenhong,et al. Synthesis Gas from Pyrolysis of Cedar Sawdust as Biomass Materials: Characterization and Catalytic Performance of Nickel-Based Monolithic Catalyst[J]. chinese journal of catalysis,2011,32(6):1017-1021. |
| APA | Lu Min,Lue Pengmei,Yuan Zhenhong,Li Huiwen,&Xu Jingliang.(2011).Synthesis Gas from Pyrolysis of Cedar Sawdust as Biomass Materials: Characterization and Catalytic Performance of Nickel-Based Monolithic Catalyst.chinese journal of catalysis,32(6),1017-1021. |
| MLA | Lu Min,et al."Synthesis Gas from Pyrolysis of Cedar Sawdust as Biomass Materials: Characterization and Catalytic Performance of Nickel-Based Monolithic Catalyst".chinese journal of catalysis 32.6(2011):1017-1021. |
入库方式： OAI收割
来源：广州能源研究所
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