Highly selective hydrogenation of furfural to furfuryl alcohol over Pt nanoparticles supported on g-C3N4 nanosheets catalysts in water
文献类型：期刊论文
| 作者 | Chen, Xiufang; Zhang, Ligang; Zhang, Bo; Guo, Xingcui; Mu, Xindong |
| 刊名 | SCIENTIFIC REPORTS
 |
| 出版日期 | 2016-06-22 |
| 卷号 | 6 |
| 英文摘要 | Graphitic carbon nitride nanosheets were investigated for developing effective Pt catalyst supports for selective hydrogenation of furfural to furfuryl alcohol in water. The nanosheets with an average thickness of about 3 nm were synthesized by a simple and green method through thermal oxidation etching of bulk g-C3N4 in air. Combined with the unique feature of nitrogen richness and locally conjugated structure, the g-C3N4 nanosheets with a high surface area of 142 m(2) g(-1) were demonstrated to be an excellent supports for loading small-size Pt nanoparticles. Superior furfural hydrogenation activity in water with complete conversion of furfural and high selectivity of furfuryl alcohol (> 99%) was observed for g-C3N4 nanosheets supported Pt catalysts. The large specific surface area, uniform dispersion of Pt nanoparticles and the stronger furfural adsorption ability of nanosheets contributed to the considerable catalytic performance. The reusability tests showed that the novel Pt catalyst could maintain high activity and stability in the furfural hydrogenation reaction. |
| WOS标题词 | Science & Technology |
| 类目[WOS] | Multidisciplinary Sciences |
| 研究领域[WOS] | Science & Technology - Other Topics |
| 关键词[WOS] | CARBON NITRIDE POLYMERS ; VISIBLE-LIGHT ; LIQUID-PHASE ; METAL NANOPARTICLES ; MILD CONDITIONS ; OXIDATION ; REDUCTION ; QUINOLINE ; CHEMICALS ; BIOMASS |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000378249900001 |
| 源URL | [http://ir.qibebt.ac.cn/handle/337004/8335]  |
| 专题 | 青岛生物能源与过程研究所_绿色化学催化团队 |
| 作者单位 | Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Key Lab Biobased Mat, Qingdao 266101, Peoples R China |
| 推荐引用方式 GB/T 7714 | Chen, Xiufang,Zhang, Ligang,Zhang, Bo,et al. Highly selective hydrogenation of furfural to furfuryl alcohol over Pt nanoparticles supported on g-C3N4 nanosheets catalysts in water[J]. SCIENTIFIC REPORTS,2016,6. |
| APA | Chen, Xiufang,Zhang, Ligang,Zhang, Bo,Guo, Xingcui,&Mu, Xindong.(2016).Highly selective hydrogenation of furfural to furfuryl alcohol over Pt nanoparticles supported on g-C3N4 nanosheets catalysts in water.SCIENTIFIC REPORTS,6. |
| MLA | Chen, Xiufang,et al."Highly selective hydrogenation of furfural to furfuryl alcohol over Pt nanoparticles supported on g-C3N4 nanosheets catalysts in water".SCIENTIFIC REPORTS 6(2016). |
入库方式： OAI收割
来源：青岛生物能源与过程研究所
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