Experimental study on hydrate-based CO2 removal from CH4/CO2 mixture
文献类型:期刊论文
作者 | Wang, Fei1,2![]() ![]() ![]() ![]() |
刊名 | ENERGY
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出版日期 | 2016-06-01 |
卷号 | 104页码:76-84 |
关键词 | CO2 removal Hydrates CH4/CO2 mixture Separation factor Multistage separation |
英文摘要 | In this work, hydrate-based CO2 removal from a CH4/CO2 mixture was studied. CH4/CO2 led to faster hydrate formation than pure CH4, because the existence of CO2 resulted in easier hydrate nucleation. Kinetic separation of CO2 was observed in the CH4/CO2 hydrate formation with different initial CO2 proportions (1.83-27.76%) due to the higher CO2 affinity of formation of hydrates. However, the initial CO2 proportion of CH4/CO2 showed no obvious effects on the hydration ratio of CH4 and CO2 and the separation efficiency when the gas was superfluous in hydrate formation. In addition, hydrate-based multistage separation of CH4/CO2 was established and conducted at different initial pressures (4, 5 and 6 MPa). The CH4 proportions were increased from 72.24% to 97.30%, 97.22% and 97.14% after separation by four, five and seven stages at initial pressures of 4, 5, and 6 MPa, respectively. (C) 2016 Elsevier Ltd. All rights reserved. |
WOS标题词 | Science & Technology ; Physical Sciences ; Technology |
类目[WOS] | Thermodynamics ; Energy & Fuels |
研究领域[WOS] | Thermodynamics ; Energy & Fuels |
关键词[WOS] | PRE-COMBUSTION CAPTURE ; CARBON-DIOXIDE ; PHASE-EQUILIBRIUM ; GAS-MIXTURES ; ENERGY EFFICIENCY ; SILICA-GEL ; METHANE ; SEPARATION ; KINETICS ; BROMIDE |
收录类别 | SCI |
语种 | 英语 |
WOS记录号 | WOS:000377727000008 |
源URL | [http://ir.qibebt.ac.cn/handle/337004/8324] ![]() |
专题 | 青岛生物能源与过程研究所_生物制氢与沼气团队 |
作者单位 | 1.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Shandong Ind Engn Lab Biogas Prod & Utilizat, Key Lab Biofuels, Qingdao 266101, Shandong, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.Guizhou Univ, Guiyang 550025, Peoples R China |
推荐引用方式 GB/T 7714 | Wang, Fei,Fu, Shanfei,Guo, Gang,et al. Experimental study on hydrate-based CO2 removal from CH4/CO2 mixture[J]. ENERGY,2016,104:76-84. |
APA | Wang, Fei,Fu, Shanfei,Guo, Gang,Jia, Zhen-Zhen,Luo, Sheng-Jun,&Guo, Rong-Bo.(2016).Experimental study on hydrate-based CO2 removal from CH4/CO2 mixture.ENERGY,104,76-84. |
MLA | Wang, Fei,et al."Experimental study on hydrate-based CO2 removal from CH4/CO2 mixture".ENERGY 104(2016):76-84. |
入库方式: OAI收割
来源:青岛生物能源与过程研究所
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