Gold-Iron Oxide Catalyst for CO Oxidation: Effect of Support Structure
文献类型:期刊论文
作者 | Cui, HZ; Guo, Y; Wang, X; Jia, CJ; Si, R |
刊名 | CATALYSTS
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出版日期 | 2016 |
卷号 | 6期号:3页码:— |
关键词 | WATER-GAS SHIFT LOW-TEMPERATURE OXIDATION AU/FE2O3 CATALYSTS CARBON-MONOXIDE DEPOSITION-PRECIPITATION AU/ALPHA-FE2O3 CATALYST NANOPARTICLES ALPHA-FE2O3 PARTICLES AU/CEO2 |
ISSN号 | 2073-4344 |
通讯作者 | Jia, CJ (reprint author), Shandong Univ, Sch Chem & Chem Engn, Key Lab Colloid & Interface Chem, Key Lab Special Aggregated Mat, Jinan 250100, Peoples R China. ; Si, R (reprint author), Chinese Acad Sci, Key Lab Interfacial Phys & Technol, Shanghai Synchrotron Radiat Facil, Shanghai Inst Appl Phys, Shanghai 201204, Peoples R China. |
英文摘要 | Gold-iron oxide (Au/FeOx) is one of the highly active catalysts for CO oxidation, and is also a typical system for the study of the chemistry of gold catalysis. In this work, two different types of iron oxide supports, i.e., hydroxylated (Fe_OH) and dehydrated iron oxide (Fe_O), have been used for the deposition of gold via a deposition-precipitation (DP) method. The structure of iron oxide has been tuned by either selecting precipitated pH of 6.7-11.2 for Fe_OH or changing calcination temperature of from 200 to 600 degrees C for Fe_O. Then, 1 wt. % Au catalysts on these iron oxide supports were measured for low-temperature CO oxidation reaction. Both fresh and used samples have been characterized by multiple techniques including transmission electron microscopy (TEM) and high-resolution TEM (HRTEM), X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS), X-ray absorption near edge structure (XANES) and temperature-programmed reduction by hydrogen (H-2-TPR). It has been demonstrated that the surface properties of the iron oxide support, as well as the metal-support interaction, plays crucial roles on the performance of Au/FeOx catalysts in CO oxidation. |
收录类别 | SCI |
语种 | 英语 |
WOS记录号 | WOS:000373798300007 |
源URL | [http://ir.sinap.ac.cn/handle/331007/25734] ![]() |
专题 | 上海应用物理研究所_中科院上海应用物理研究所2011-2017年 |
推荐引用方式 GB/T 7714 | Cui, HZ,Guo, Y,Wang, X,et al. Gold-Iron Oxide Catalyst for CO Oxidation: Effect of Support Structure[J]. CATALYSTS,2016,6(3):—. |
APA | Cui, HZ,Guo, Y,Wang, X,Jia, CJ,&Si, R.(2016).Gold-Iron Oxide Catalyst for CO Oxidation: Effect of Support Structure.CATALYSTS,6(3),—. |
MLA | Cui, HZ,et al."Gold-Iron Oxide Catalyst for CO Oxidation: Effect of Support Structure".CATALYSTS 6.3(2016):—. |
入库方式: OAI收割
来源:上海应用物理研究所
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