Nitrogen, Phosphorus, and Sulfur Co-Doped Hollow Carbon Shell as Superior Metal-Free Catalyst for Selective Oxidation of Aromatic Alkanes
文献类型：期刊论文
| 作者 | Yang, Shuliang1; Peng, Li2; Huang, Peipei1; Wang, Xiaoshi1; Sun, Yongbin1; Cao, Changyan1; Song, Weiguo1 |
| 刊名 | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
 |
| 出版日期 | 2016-03-14 |
| 卷号 | 55期号:12页码:4016-4020 |
| 关键词 | carbon doping heterogeneous catalysis metal-free catalysts selective oxidation |
| 英文摘要 | Metal-free heteroatom-doped carbocatalysts with a high surface area are desirable for catalytic reactions. In this study, we found an efficient strategy to prepare nitrogen, phosphorus, and sulfur co-doped hollow carbon shells (denote as NPS-HCS) with a surface area of 1020m(2)g(-1). Using a poly(cyclotriphosphazene-co-4,4-sulfonyldiphenol) (PZS) shell as carbon source and N, P, S-doping source, and the ZIF-67 core as structural template as well as extra N-doping source, NPS-HCS were obtained with a high surface area and superhydrophilicity. All these features render the prepared NPS-HCS a superior metal-free carbocatalyst for the selective oxidation of aromatic alkanes in aqueous solution. This study provides a reliable and facile route to prepare doped carbocatalysts with enhanced catalytic properties. |
| 收录类别 | SCI ; CCR |
| 语种 | 英语 |
| 源URL | [http://ir.iccas.ac.cn/handle/121111/35959]  |
| 专题 | 化学研究所_分子纳米结构与纳米技术实验室 |
| 作者单位 | 1.Chinese Acad Sci, Inst Chem, Lab Mol Nanostruct & Nanotechnol, Beijing Natl Lab Mol Sci, Beijing 100190, Peoples R China 2.EPFL, EPFL ISIC Valais, Inst Chem Sci & Engn, CH-1950 Sion, Switzerland |
| 推荐引用方式 GB/T 7714 | Yang, Shuliang,Peng, Li,Huang, Peipei,et al. Nitrogen, Phosphorus, and Sulfur Co-Doped Hollow Carbon Shell as Superior Metal-Free Catalyst for Selective Oxidation of Aromatic Alkanes[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2016,55(12):4016-4020. |
| APA | Yang, Shuliang.,Peng, Li.,Huang, Peipei.,Wang, Xiaoshi.,Sun, Yongbin.,...&Song, Weiguo.(2016).Nitrogen, Phosphorus, and Sulfur Co-Doped Hollow Carbon Shell as Superior Metal-Free Catalyst for Selective Oxidation of Aromatic Alkanes.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,55(12),4016-4020. |
| MLA | Yang, Shuliang,et al."Nitrogen, Phosphorus, and Sulfur Co-Doped Hollow Carbon Shell as Superior Metal-Free Catalyst for Selective Oxidation of Aromatic Alkanes".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 55.12(2016):4016-4020. |
入库方式： OAI收割
来源：化学研究所
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