Rational design and electron transfer kinetics of MoS2/CdS nanodots-on-nanorods for efficient visible-light-driven hydrogen generation
文献类型：期刊论文
| 作者 | Yin, Xing-Liang1,3; He, Gui-Ying2,3; Sun, Bing1,3; Jiang, Wen-Jie1,3; Xue, Ding-Jiang1,3; Xia, An-Dong2,3; Wan, Li-Jun1,3; Hu, Jin-Song1,3 |
| 刊名 | NANO ENERGY
 |
| 出版日期 | 2016-10-01 |
| 卷号 | 28页码:319-329 |
| 关键词 | Nano structures Water splitting Hetero structures HER Hydrogen evolution |
| 英文摘要 | The efficiency of CdS-based photocatalysts for H-2 evolution is limited by the ultrafast charge recombination. Here, we demonstrated the one-pot synthesis of a novel MoS2/CdS photocatalyst with the structure of partially crystalline MoS2 nanodots growing on single-crystalline CdS nanorods. This heterostructure not only effectively reduces the bulk and surface charge recombination owing to single crystalline CdS nanorod matrix and efficient electron transfer, also provides plenty of active sites for hydrogen evolution reaction (HER) and accessible room for prompt hole extraction. The femtosecond transient absorption (TA) analysis reveals the effective electron transfer from CdS to MoS2 in similar to 20 ps. As a result, MoS2/CdS exhibits extraordinary photocatalytic activity with a H-2 evolution rate of 60.28 mmol/g/h under visible light irradiation, far exceeding all previous HER photocatalysts with MoS2 as cocatalysts. (C) 2016 Published by Elsevier Ltd. |
| 收录类别 | SCI |
| 语种 | 英语 |
| 源URL | [http://ir.iccas.ac.cn/handle/121111/35652]  |
| 专题 | 化学研究所_光化学实验室 |
| 作者单位 | 1.Chinese Acad Sci, Inst Chem, Key Lab Mol Nanostruct & Nanotechnol, Beijing Natl Lab Mol Sci, 2 North First St, Beijing 100190, Peoples R China 2.Chinese Acad Sci, Inst Chem, Key Lab Photochem, Beijing Natl Lab Mol Sci, 2 North First St, Beijing 100190, Peoples R China 3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Yin, Xing-Liang,He, Gui-Ying,Sun, Bing,et al. Rational design and electron transfer kinetics of MoS2/CdS nanodots-on-nanorods for efficient visible-light-driven hydrogen generation[J]. NANO ENERGY,2016,28:319-329. |
| APA | Yin, Xing-Liang.,He, Gui-Ying.,Sun, Bing.,Jiang, Wen-Jie.,Xue, Ding-Jiang.,...&Hu, Jin-Song.(2016).Rational design and electron transfer kinetics of MoS2/CdS nanodots-on-nanorods for efficient visible-light-driven hydrogen generation.NANO ENERGY,28,319-329. |
| MLA | Yin, Xing-Liang,et al."Rational design and electron transfer kinetics of MoS2/CdS nanodots-on-nanorods for efficient visible-light-driven hydrogen generation".NANO ENERGY 28(2016):319-329. |
入库方式： OAI收割
来源：化学研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。