Nanoscale imaging of Li and B in nuclear waste glass, a comparison of ToF-SIMS, NanoSIMS, and APT
文献类型：期刊论文
| 作者 | Wang, Zhaoying1,2; Liu, Jia2; Zhou, Yufan2,3,4; Neeway, James J.5; Schreiber, Daniel K.5; Crum, Jarrod V.5; Ryan, Joseph V.5; Wang, Xue-Lin3,4; Wang, Fuyi1; Zhu, Zihua2 |
| 刊名 | SURFACE AND INTERFACE ANALYSIS
 |
| 出版日期 | 2016-12-01 |
| 卷号 | 48期号:13页码:1392-1401 |
| 关键词 | ToF-SIMS NanoSIMS APT nanoscale imaging lithium boron nuclear waste glass |
| 英文摘要 | It has been very difficult to use popular elemental imaging techniques to image Li and B distribution in glass samples with nanoscale resolution. In this study, time-of-flight secondary ion mass spectrometry, nanoscale secondary ion mass spectrometry, and atom probe tomography (APT) were used to image the distribution of Li and B in two representative glass samples, and their performance was comprehensively compared. APT can provide three-dimensional Li and B imaging with very high spatial resolution (2nm). In addition, absolute quantification of Li and B is possible, although there remains room for improving accuracy. However, the major drawbacks of APT include poor sample compatibility and limited field of view (normally 100x100x500nm(3)). Comparatively, time-of-flight secondary ion mass spectrometry and nanoscale secondary ion mass spectrometry are sample-friendly with flexible field of view (up to 500x500 mu m(2) and image stitching is feasible); however, lateral resolution is limited to only about 100nm. Therefore, secondary ion mass spectrometry and APT can be regarded as complementary techniques for nanoscale imaging of Li and B in glass and other novel materials. Copyright (c) 2016 John Wiley & Sons, Ltd. |
| 收录类别 | SCI |
| 语种 | 英语 |
| 源URL | [http://ir.iccas.ac.cn/handle/121111/35719]  |
| 专题 | 化学研究所_活体分析化学实验室 |
| 作者单位 | 1.Chinese Acad Sci, Beijing Ctr Mass Spectrometry, CAS Key Lab Analyt Chem Living Biosyst, Beijing Natl Lab Mol Sci,Inst Chem, Beijing 100190, Peoples R China 2.Pacific Northwest Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA 3.Shandong Univ, Sch Phys, State Key Lab Crystal Mat, Jinan 250100, Peoples R China 4.Shandong Univ, Key Lab Particle Phys & Particle Irradiat MOE, Jinan 250100, Peoples R China 5.Pacific Northwest Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA |
| 推荐引用方式 GB/T 7714 | Wang, Zhaoying,Liu, Jia,Zhou, Yufan,et al. Nanoscale imaging of Li and B in nuclear waste glass, a comparison of ToF-SIMS, NanoSIMS, and APT[J]. SURFACE AND INTERFACE ANALYSIS,2016,48(13):1392-1401. |
| APA | Wang, Zhaoying.,Liu, Jia.,Zhou, Yufan.,Neeway, James J..,Schreiber, Daniel K..,...&Zhu, Zihua.(2016).Nanoscale imaging of Li and B in nuclear waste glass, a comparison of ToF-SIMS, NanoSIMS, and APT.SURFACE AND INTERFACE ANALYSIS,48(13),1392-1401. |
| MLA | Wang, Zhaoying,et al."Nanoscale imaging of Li and B in nuclear waste glass, a comparison of ToF-SIMS, NanoSIMS, and APT".SURFACE AND INTERFACE ANALYSIS 48.13(2016):1392-1401. |
入库方式： OAI收割
来源：化学研究所
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