Graphene oxide/carbon nanotubes-Fe3O4 supported Pd nanoparticles for hydrogenation of nitroarenes and C-H activation
文献类型:期刊论文
作者 | Yang, Fan1; Feng, Andong1; Wang, Chunxia2; Dong, Sen1; Chi, Cheng1; Jia, Xilai1; Zhang, Liqiang1; Li, Yongfeng1 |
刊名 | RSC ADVANCES
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出版日期 | 2016 |
卷号 | 6期号:21页码:16911-16916 |
英文摘要 | Fe3O4 magnetic nanocomposites combined with graphene oxide (GO) and carbon nanotubes (CNTs) are synthesized by a hydrothermal method, followed by synthesis of GO/CNT-Fe3O4 supported Pd nanoparticles using a gas-liquid interfacial plasma (GLIP) method with Pd(OAc)(2) as a precursor, and the Pd nanoparticles show a uniform particle size distribution. The catalysts exhibit remarkable catalytic activity during the hydrogenation of nitroarenes under H-2 atmosphere at 60 degrees C in water using a small amount of catalyst, and the catalyst can be magnetically separated from the reaction mixture. The addition of the Fe3O4 component to the GO/CNTs can be used to effectively prevent aggregation and restacking of GO and the CNTs, and the GO/CNT composite can adjust the hydrophilic-hydrophobic property of the catalysts. Furthermore, the Pd catalyst can be readily recovered and reused several times without a significant decrease in activity. It is worth mentioning that the Pd-3 catalysts show remarkable activity during C-H functionalization. |
收录类别 | SCI |
语种 | 英语 |
源URL | [http://ir.iccas.ac.cn/handle/121111/35875] ![]() |
专题 | 化学研究所_活体分析化学实验室 |
作者单位 | 1.China Univ Petr, State Key Lab Heavy Oil Proc, Beijing 102249, Peoples R China 2.Chinese Acad Sci, Inst Chem, Key Lab Analyt Chem Living Biosyst, Beijing Natl Lab Mol Sci, Beijing 100190, Peoples R China |
推荐引用方式 GB/T 7714 | Yang, Fan,Feng, Andong,Wang, Chunxia,et al. Graphene oxide/carbon nanotubes-Fe3O4 supported Pd nanoparticles for hydrogenation of nitroarenes and C-H activation[J]. RSC ADVANCES,2016,6(21):16911-16916. |
APA | Yang, Fan.,Feng, Andong.,Wang, Chunxia.,Dong, Sen.,Chi, Cheng.,...&Li, Yongfeng.(2016).Graphene oxide/carbon nanotubes-Fe3O4 supported Pd nanoparticles for hydrogenation of nitroarenes and C-H activation.RSC ADVANCES,6(21),16911-16916. |
MLA | Yang, Fan,et al."Graphene oxide/carbon nanotubes-Fe3O4 supported Pd nanoparticles for hydrogenation of nitroarenes and C-H activation".RSC ADVANCES 6.21(2016):16911-16916. |
入库方式: OAI收割
来源:化学研究所
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