Electrochemical reduction of CO2 to CO using graphene oxide/carbon nanotube electrode in ionic liquid/acetonitrile system
文献类型:期刊论文
作者 | Zhu, Qinggong; Ma, Jun; Kang, Xinchen; Sun, Xiaofu; Hu, Jiayin; Yang, Guanying; Han, Buxing1 |
刊名 | SCIENCE CHINA-CHEMISTRY
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出版日期 | 2016-05-01 |
卷号 | 59期号:5页码:551-556 |
关键词 | carbon dioxide electrochemical reduction carbon monoxide electrophoretic deposition carbon based materials |
英文摘要 | Electrochemical reduction of CO2 to CO is an interesting topic. In this work, we prepared metal-free electrodes by depositing graphene oxide (GO), multi-walled carbon nanotube (MWCNT), and GO/MWCNT composites on carbon paper (CP) using electrophoretic deposition (EPD) method. The electrodes were characterized by different methods, such as X-ray diffraction (XRD) and X-ray photoelectron spectroscopy (XPS). The electrochemical reduction of CO2 to CO was conducted on the electrodes in 1-butyl-3-methylimidazolium tetrafluoroborate ([Bmim]BF4)/acetonitrile (MeCN) electrolyte, and the composition of the electrolyte influenced the reaction significantly. It was demonstrated that GO/MWCNT-CP electrode was very effective for the reaction in IL (90 wt%)/MeCN binary mixture, the Faradaic efficiency of CO and current density were even higher than those on Au and Ag electrodes in the same electrolyte. |
收录类别 | SCI |
语种 | 英语 |
源URL | [http://ir.iccas.ac.cn/handle/121111/36076] ![]() |
专题 | 化学研究所_胶体、界面与化学热力学实验室 |
作者单位 | 1.Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, Beijing 100190, Peoples R China 2.Chinese Acad Sci, Inst Chem, CAS Key Lab Colloid Interface & Chem Thermodynam, Beijing 100190, Peoples R China |
推荐引用方式 GB/T 7714 | Zhu, Qinggong,Ma, Jun,Kang, Xinchen,et al. Electrochemical reduction of CO2 to CO using graphene oxide/carbon nanotube electrode in ionic liquid/acetonitrile system[J]. SCIENCE CHINA-CHEMISTRY,2016,59(5):551-556. |
APA | Zhu, Qinggong.,Ma, Jun.,Kang, Xinchen.,Sun, Xiaofu.,Hu, Jiayin.,...&Han, Buxing.(2016).Electrochemical reduction of CO2 to CO using graphene oxide/carbon nanotube electrode in ionic liquid/acetonitrile system.SCIENCE CHINA-CHEMISTRY,59(5),551-556. |
MLA | Zhu, Qinggong,et al."Electrochemical reduction of CO2 to CO using graphene oxide/carbon nanotube electrode in ionic liquid/acetonitrile system".SCIENCE CHINA-CHEMISTRY 59.5(2016):551-556. |
入库方式: OAI收割
来源:化学研究所
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