中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Minimum Thermal Conductivity in Weak Topological Insulators with Bismuth-Based Stack Structure

文献类型:期刊论文

作者Wei, Ping1,2; Yang, Jiong1,3; Guo, Liang4,5; Wang, Shanyu1; Wu, Lihua1,3; Xu, Xianfan4,5; Zhao, Wenyu2; Zhang, Qingjie2; Zhang, Wenqing3,6; Dresselhaus, Mildred S.7
刊名ADVANCED FUNCTIONAL MATERIALS
出版日期2016-08-02
卷号26期号:29页码:5360-5367
英文摘要Contrary to the conventional belief that the consideration for topological insulators (TIs) as potential thermoelectrics is due to their excellent electrical properties benefiting from the topological surface states, this work shows that the 3D weak TIs, formed by alternating stacks of quantum spin Hall layers and normal insulator (NI) layers, can also be decent thermoelectrics because of their focus on minimum thermal conductivity. The minimum lattice thermal conductivity is experimentally confirmed in Bi14Rh3I9 and theoretically predicted for Bi2TeI at room temperature. It is revealed that the topologically "trivial" NI layers play a surprisingly critical role in hindering phonon propagation. The weak bonding in the NI layers gives rise to significantly low sound velocity, and the localized low-frequency vibrations of the NI layers cause strong acoustic-optical interactions and lattice anharmonicity. All these features are favorable for the realization of exceptionally low lattice thermal conductivity, and therefore present remarkable opportunities for developing high-performance thermoelectrics in weak TIs.
WOS标题词Science & Technology ; Physical Sciences ; Technology
类目[WOS]Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
研究领域[WOS]Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
关键词[WOS]AUGMENTED-WAVE METHOD ; SINGLE DIRAC CONE ; THERMOELECTRIC-MATERIALS ; BI2TE3 ; PERFORMANCE ; EFFICIENCY ; CRYSTALS ; BEHAVIOR ; SURFACE ; ORIGIN
收录类别SCI
语种英语
WOS记录号WOS:000382548000021
源URL[http://ir.sic.ac.cn/handle/331005/22126]  
专题上海硅酸盐研究所_高性能陶瓷和超微结构国家重点实验室_期刊论文
作者单位1.Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USA
2.Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, Wuhan 430070, Peoples R China
3.Shanghai Univ, Mat Genome Inst, Shanghai 200444, Peoples R China
4.Purdue Univ, Sch Mech Engn, W Lafayette, IN 47907 USA
5.Purdue Univ, Birck Nanotechnol Ctr, W Lafayette, IN 47907 USA
6.Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine, Shanghai 200050, Peoples R China
7.MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA
推荐引用方式
GB/T 7714
Wei, Ping,Yang, Jiong,Guo, Liang,et al. Minimum Thermal Conductivity in Weak Topological Insulators with Bismuth-Based Stack Structure[J]. ADVANCED FUNCTIONAL MATERIALS,2016,26(29):5360-5367.
APA Wei, Ping.,Yang, Jiong.,Guo, Liang.,Wang, Shanyu.,Wu, Lihua.,...&Yang, Jihui.(2016).Minimum Thermal Conductivity in Weak Topological Insulators with Bismuth-Based Stack Structure.ADVANCED FUNCTIONAL MATERIALS,26(29),5360-5367.
MLA Wei, Ping,et al."Minimum Thermal Conductivity in Weak Topological Insulators with Bismuth-Based Stack Structure".ADVANCED FUNCTIONAL MATERIALS 26.29(2016):5360-5367.

入库方式: OAI收割

来源:上海硅酸盐研究所

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