Growth of Horizontal Semiconducting SWNT Arrays with Density Higher than 100 tubes/mu m using Ethanol/Methane Chemical Vapor Deposition
文献类型:期刊论文
作者 | Kang, LX(康黎星); Zhang, SC; Li, QW(李清文); Zhang, J |
刊名 | JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
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出版日期 | 2016 |
卷号 | 138期号:21 |
通讯作者 | Zhang, J |
英文摘要 | Horizontally aligned semiconducting single walled carbon nanotube (s-SWNT) arrays with a certain density are highly desirable for future electronic devices. However, obtaining s-SWNT arrays with simultaneously high purity and high density is extremely challenging. We report herein a rational approach, using ethanol/methane chemical vapor deposition, to grow SWNT arrays with a s-SWNT ratio over 91% and a density higher than 100 tubes/mu m. In this approach, at a certain temperature, ethanol was fully thermally decomposed to feed carbon atoms for Trojan-Mo catalysts growing high density SWNT arrays, while the incomplete pyrolysis of methane provided appropriate active H radicals with the help of catalytic sapphire surface to inhibit metallic SWNT (m-SWNT) growth. The synergistic effect of ethanol/methane mixtures resulted in enriched semiconducting SWNTs and no obvious decrease in nanotube density due to their milder reactivity and higher controllability at suitable growth conditions. This work represents a step forward in large-area synthesis of high density s-SWNT arrays on substrates and demonstrates potential applications in scalable carbon nanotube electronics. |
关键词[WOS] | WALLED CARBON NANOTUBES ; TRANSISTORS |
收录类别 | SCI ; EI |
语种 | 英语 |
WOS记录号 | WOS:000377151400009 |
源URL | [http://ir.sinano.ac.cn/handle/332007/4827] ![]() |
专题 | 苏州纳米技术与纳米仿生研究所_先进材料研究部_李清文团队 |
推荐引用方式 GB/T 7714 | Kang, LX,Zhang, SC,Li, QW,et al. Growth of Horizontal Semiconducting SWNT Arrays with Density Higher than 100 tubes/mu m using Ethanol/Methane Chemical Vapor Deposition[J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,2016,138(21). |
APA | Kang, LX,Zhang, SC,Li, QW,&Zhang, J.(2016).Growth of Horizontal Semiconducting SWNT Arrays with Density Higher than 100 tubes/mu m using Ethanol/Methane Chemical Vapor Deposition.JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,138(21). |
MLA | Kang, LX,et al."Growth of Horizontal Semiconducting SWNT Arrays with Density Higher than 100 tubes/mu m using Ethanol/Methane Chemical Vapor Deposition".JOURNAL OF THE AMERICAN CHEMICAL SOCIETY 138.21(2016). |
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