Hydrogen-rich gas production by steam gasification of hydrochar derived from sewage sludge
文献类型:期刊论文
作者 | Gai, Chao; Guo, Yanchuan; Liu, Tingting; Peng, Nana; Liu, Zhengang |
刊名 | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
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出版日期 | 2016-02-09 |
卷号 | 41期号:5页码:3363-3372 |
关键词 | Sewage sludge Gasification Steam Alkali catalyst Hydrogen Hydrothermal carbonization |
英文摘要 | Hydrothermal carbonization is an effective pretreatment for further thermal conversion of high moisture biomass without a high cost of a dehydration process. The current paper concerns the properties of hydrochar derived from hydrothermal carbonization of sewage sludge, and the feasibility of steam gasification of hydrochar for hydrogen-rich gas production was investigated. Sewage sludge derived hydrochar was characterized using scanning electron microscopy, Fourier transform infrared spectroscopy, and inductively coupled plasma atomic emission spectroscopy to evaluate its feasibility for gasification application. The effect of reaction temperature, steam to biomass mass ratio, and addition of alkali catalysts on steam gasification characteristics of raw sewage sludge and corresponding hydrochar were evaluated, in terms of major composition of the produced gas, gas yield, gasification efficiency and energy density. The results showed that sewage sludge derived hydrochar was rich in hydrophilic functional groups and increased Fe, Ni, alkali and alkaline earth metals (i.e. K, Na, Ca, Mg), resulting in a higher hydrogen yield and energy efficiency than direct steam gasification of sewage sludge under identical conditions. In addition, hydrogen-rich gas production was also favored with the presence of alkali catalysts, especially for the hydrochar. The present study demonstrates that hydrothermal carbonization provides an effective pretreatment of sewage sludge for production of hydrogen-rich gas via steam gasification. Copyright (C) 2016, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. |
收录类别 | SCI |
源URL | [http://ir.rcees.ac.cn/handle/311016/35783] ![]() |
专题 | 生态环境研究中心_固体废弃物处理与资源化实验室 |
推荐引用方式 GB/T 7714 | Gai, Chao,Guo, Yanchuan,Liu, Tingting,et al. Hydrogen-rich gas production by steam gasification of hydrochar derived from sewage sludge[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2016,41(5):3363-3372. |
APA | Gai, Chao,Guo, Yanchuan,Liu, Tingting,Peng, Nana,&Liu, Zhengang.(2016).Hydrogen-rich gas production by steam gasification of hydrochar derived from sewage sludge.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,41(5),3363-3372. |
MLA | Gai, Chao,et al."Hydrogen-rich gas production by steam gasification of hydrochar derived from sewage sludge".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 41.5(2016):3363-3372. |
入库方式: OAI收割
来源:生态环境研究中心
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