Characterization of Perovskite Obtained from Two-Step Deposition on Mesoporous Titania
文献类型：期刊论文
| 作者 | Chen, Shanshan1; Lei, Lei2,3; Yang, Songwang2; Liu, Yan2; Wang, Zhong-Sheng1 |
| 刊名 | ACS APPLIED MATERIALS & INTERFACES
 |
| 出版日期 | 2015-11-25 |
| 卷号 | 7期号:46页码:25770-25776 |
| 关键词 | crystal growth engineering energy level light harvesting pervoskite solar cell time resolved photoluminescene decay |
| 英文摘要 | The properties of perovskite films are sensitive to the fabrication method, which plays a crucial role in the performance of perovskite solar cell. In this work, we fabricate organo-lead iodide perovskite on mesoporous TiO2 films through two different two-step deposition methods, respectively, for the purpose of studying the crystal growth of perovskite film and its effect on light harvesting efficiency, defect density, charge extraction rate, and energy levels. The crystal growth exerts a significant influence on the morphology and hence the film properties, which are found to correlate with the performance of solar cells. It is found that vapor deposition of methylammonium iodide in the PbI2 lattice gives a more complete coverage on mesoporous TiO2 with a flatter surface and Fermi level closer to the middle of the band-gap, resulting in higher light absorption in the visible spectral region, lower defect density, and faster charge extraction, as compared to the sequential solution deposition. For this reason, the vapor-processed perovskite film achieves higher short-circuit photocurrent and power conversion efficiency than the solution-processed film. |
| WOS标题词 | Science & Technology ; Technology |
| 类目[WOS] | Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary |
| 研究领域[WOS] | Science & Technology - Other Topics ; Materials Science |
| 关键词[WOS] | ORGANOMETAL HALIDE PEROVSKITES ; SENSITIZED SOLAR-CELLS ; SEQUENTIAL DEPOSITION ; THIN-FILM ; DIFFUSION LENGTHS ; EFFICIENT ; HYSTERESIS ; CH3NH3PBI3 ; INTERFACE ; ABSORBER |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000366005600028 |
| 源URL | [http://ir.sic.ac.cn/handle/331005/23386]  |
| 专题 | 上海硅酸盐研究所_能量转换材料重点实验室_期刊论文 |
| 作者单位 | 1.Fudan Univ, Collaborat Innovat Ctr Chem Energy Mat, Dept Chem, Adv Mat Lab, Shanghai 200438, Peoples R China 2.Chinese Acad Sci, Key Lab Mat Energy Convers, Shanghai 200050, Peoples R China 3.Univ Chinese Acad Sci, Beijing 100039, Peoples R China |
| 推荐引用方式 GB/T 7714 | Chen, Shanshan,Lei, Lei,Yang, Songwang,et al. Characterization of Perovskite Obtained from Two-Step Deposition on Mesoporous Titania[J]. ACS APPLIED MATERIALS & INTERFACES,2015,7(46):25770-25776. |
| APA | Chen, Shanshan,Lei, Lei,Yang, Songwang,Liu, Yan,&Wang, Zhong-Sheng.(2015).Characterization of Perovskite Obtained from Two-Step Deposition on Mesoporous Titania.ACS APPLIED MATERIALS & INTERFACES,7(46),25770-25776. |
| MLA | Chen, Shanshan,et al."Characterization of Perovskite Obtained from Two-Step Deposition on Mesoporous Titania".ACS APPLIED MATERIALS & INTERFACES 7.46(2015):25770-25776. |
入库方式： OAI收割
来源：上海硅酸盐研究所
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