Promotional effect of colloidal alumina on the activity of the In/HZSM-5 catalyst for the selective reduction of NO with methane
文献类型:期刊论文
作者 | Ren, LL; Zhang, T; Tang, JW; Zhao, JF; Li, N; Lin, LW |
刊名 | applied catalysis b-environmental
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出版日期 | 2003-03-10 |
卷号 | 41期号:1-2页码:129-136 |
关键词 | DeNO(x) SCR of NOx methane In/HZSM-5 Al2O3 Co-operative effect |
产权排序 | 1;1 |
英文摘要 | colloidal alumina was used to improve the activity of an in/hzsm-5 catalyst for the selective reduction of no with ch4 in the excess of oxygen. compared with in/hzsm-5, the in/hzsm-5/al2o3 catalyst showed higher activity in a wide range of reaction temperatures. it is visualized that a synergetic effect between in/hzsm-5 and al2o3 enhances the conversion of nox. the addition of al2o3 improved the conversion of no to no2 and facilitated the activation of methane. an in/hzsm-5/al2o3 pre-treated with steam for 15 h at 700 degreesc still showed a high activity for the removal of nox with methane, while an in/hzsm-5 similarly pre-treated with steam showed a lower activity than the fresh sample. the activity of the in/hzsm-5/al2o3 catalyst could be restored completely after water vapor was removed from the feed gas. furthermore, it was found that the in/hzsm-5/al2o3 remained fairly active under high ghsv and o-2 concentration conditions. it was also interesting to find that an increase in no content could enhance the conversion of methane, and this illustrates that the existence of no is beneficial for the activation of methane. (c) 2002 elsevier science b.v. all rights reserved. |
WOS标题词 | science & technology ; physical sciences ; technology |
类目[WOS] | chemistry, physical ; engineering, environmental ; engineering, chemical |
研究领域[WOS] | chemistry ; engineering |
关键词[WOS] | nitrogen monoxide ; zeolite catalysts ; excess oxygen ; nitric-oxide ; gallium ; indium ; atmosphere ; platinum ; sites ; ch4 |
收录类别 | ISTP ; SCI |
原文出处 | true |
语种 | 英语 |
WOS记录号 | WOS:000181679800012 |
公开日期 | 2010-11-30 |
源URL | [http://159.226.238.44/handle/321008/82483] ![]() |
专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
作者单位 | Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China |
推荐引用方式 GB/T 7714 | Ren, LL,Zhang, T,Tang, JW,et al. Promotional effect of colloidal alumina on the activity of the In/HZSM-5 catalyst for the selective reduction of NO with methane[J]. applied catalysis b-environmental,2003,41(1-2):129-136. |
APA | Ren, LL,Zhang, T,Tang, JW,Zhao, JF,Li, N,&Lin, LW.(2003).Promotional effect of colloidal alumina on the activity of the In/HZSM-5 catalyst for the selective reduction of NO with methane.applied catalysis b-environmental,41(1-2),129-136. |
MLA | Ren, LL,et al."Promotional effect of colloidal alumina on the activity of the In/HZSM-5 catalyst for the selective reduction of NO with methane".applied catalysis b-environmental 41.1-2(2003):129-136. |
入库方式: OAI收割
来源:大连化学物理研究所
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