Spectral modulation observed in artificial photosynthetic complexes by real-time vibrational spectroscopy
文献类型：期刊论文
| 作者 | Leng, Yuxin; Du, Juan; Yuan, Wei; Xing, Xin; Miyatake, Tomohiro; Tamiaki, Hitoshi; Kobayashi, Takayoshi |
| 刊名 | Chem. Phys. Lett.
 |
| 出版日期 | 2017 |
| 卷号 | 683页码:154 |
| 通讯作者 | kobayashi@ils.uec.ac.jp ; lengyuxin@mail.siom.ac.cn |
| 英文摘要 | By real-time vibrational spectroscopy using 6.8 fs pulses, real-time vibronic coupling in stair-like zinc chlorin aggregates was studied. Besides the observed fast excitonic relaxation, amplitudes of coherent molecular vibrations are found to be linearly dispersed from the resonant peak as a function of their own vibrational frequencies. In addition, the initial phases of the molecular vibrations exhibiting clear pi phase jump have been observed. All these results indicate that coherent vibrations in the artificial chlorosome intermediate energy exchange between the laser fields around the resonant peak and those separated from it by photon energy equal to the vibrational frequencies. |
| 收录类别 | SCI |
| 资助信息 | 100 Talents Program of Chinese Academy of Sciences (CAS), Strategic Priority Research Program of CAS [XDB1603, 61475169, 61521093, 11127901]; Japan Science and Technology |
| WOS记录号 | WOS:000405802200024 |
| 源URL | [http://ir.siom.ac.cn/handle/181231/28718]  |
| 专题 | 上海光学精密机械研究所_强场激光物理国家重点实验室 |
| 作者单位 | 中国科学院上海光学精密机械研究所 |
| 推荐引用方式 GB/T 7714 | Leng, Yuxin,Du, Juan,Yuan, Wei,et al. Spectral modulation observed in artificial photosynthetic complexes by real-time vibrational spectroscopy[J]. Chem. Phys. Lett.,2017,683:154. |
| APA | Leng, Yuxin.,Du, Juan.,Yuan, Wei.,Xing, Xin.,Miyatake, Tomohiro.,...&Kobayashi, Takayoshi.(2017).Spectral modulation observed in artificial photosynthetic complexes by real-time vibrational spectroscopy.Chem. Phys. Lett.,683,154. |
| MLA | Leng, Yuxin,et al."Spectral modulation observed in artificial photosynthetic complexes by real-time vibrational spectroscopy".Chem. Phys. Lett. 683(2017):154. |
入库方式： OAI收割
来源：上海光学精密机械研究所
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