中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
A Novel Cathode Architecture Using Ordered Pt Nanostructure Thin Film for AAEMFC Application

文献类型:期刊论文

作者Song, Wei2; Jia, Jia1,2; Yu, Hongmei2; Gao, Xueqiang1,2; Fu, Li1,2; Shao, Zhigang2; Chi, Jun1,2; Yi, Baolian2
刊名ELECTROCHIMICA ACTA
出版日期2016-12-01
卷号220页码:67-74
关键词alkaline anion-exchange membrane fuel cells membrane electrode assembly ordered catalyst layer nanostructure thin film arrays
英文摘要A novel cathode architecture using vertically aligned Co-OH-CO3 nanoneedle arrays as ordered catalyst support for AAEMFC application is developed. Co-OH-CO3 nanoneedle arrays are directly grown on a stainless steel sheet via hydrothermal reaction. A Pt nanosturcture thin film is prepared on the surface of Co-OH-CO3 by sputter deposition to form Pt/Co-OH-CO3 nanoneedle arrays and the thickness of the Pt nanostructure thin film is only several nanometers. After transferring the Pt/Co-OH-CO3 nanoneedle arrays on an alkaline anion exchange membrane by hot pressing and acid washing, the novel cathode catalyst layer is formed, with the thickness of several hundred nanometers. Without alkaline ionomer in the cathode catalyst layer and the AAEMFC with the prepared MEA shows a peak power density of 113 mW cm(-2) with ultra-low Pt loading down to 20 mu g cm(-2). This is the first time that order-structured electrode architecture is applied in the AAEMFC, which can deliver higher power density without alkaline ionomer than the conventional MEA with the same Pt loading. (C) 2016 Elsevier Ltd. All rights reserved.
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Electrochemistry
关键词[WOS]MEMBRANE FUEL-CELLS ; ALKALINE POLYMER ELECTROLYTE ; HYDROGEN OXIDATION REACTION ; ANION-EXCHANGE MEMBRANE ; PERFORMANCE ; CATALYSTS ; IONOMER ; ELECTROCATALYSTS
收录类别SCI
语种英语
WOS记录号WOS:000389090800008
源URL[http://cas-ir.dicp.ac.cn/handle/321008/150347]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, Grad Sch, Beijing 100039, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, Fuel Cell Syst & Engn Lab, 457 Zhongshan Rd, Dalian 116023, Peoples R China
推荐引用方式
GB/T 7714
Song, Wei,Jia, Jia,Yu, Hongmei,et al. A Novel Cathode Architecture Using Ordered Pt Nanostructure Thin Film for AAEMFC Application[J]. ELECTROCHIMICA ACTA,2016,220:67-74.
APA Song, Wei.,Jia, Jia.,Yu, Hongmei.,Gao, Xueqiang.,Fu, Li.,...&Yi, Baolian.(2016).A Novel Cathode Architecture Using Ordered Pt Nanostructure Thin Film for AAEMFC Application.ELECTROCHIMICA ACTA,220,67-74.
MLA Song, Wei,et al."A Novel Cathode Architecture Using Ordered Pt Nanostructure Thin Film for AAEMFC Application".ELECTROCHIMICA ACTA 220(2016):67-74.

入库方式: OAI收割

来源:大连化学物理研究所

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