Low-temperature H-2-plasma-assisted NOx storage and reduction over a combined Pt/Ba/Al and LaMnFe catalyst
文献类型:期刊论文
作者 | Li, Ming-run2; Crocker, Mark3; Zhang, Zhao-shun1,4; Shi, Chuan1; Bai, Zhi-feng1; Chen, Bing-bing1 |
刊名 | CATALYSIS SCIENCE & TECHNOLOGY
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出版日期 | 2017 |
卷号 | 7期号:1页码:145-158 |
英文摘要 | A model catalyst of the Pt/Ba/Al2O3 (PBA) type exhibited poor activity in NOx storage-reduction (NSR) at low temperatures (<= 300 degrees C) even under a plasma-enhanced process. In order to achieve optimal NOx removal efficiency during plasma-assisted NOx storage-reduction in the presence of H2O and CO2, a PBA+LMF (LaMn0.9Fe0.1O3) catalyst was prepared by mechanical mixing. Compared to the PBA and LMF references, the combined PBA+LMF catalyst showed an obvious synergistic effect with respect to NOx storage capacity. With the assistance of H-2 plasma in rich phase, higher NOx conversions could be obtained over the PBA+LMF sample over a wide temperature range (200-350 degrees C). The origin of the synergy was clarified on the basis of structure-activity correlations. The combination of non-thermal plasma and heterogeneous catalysis was proven to be very effective in improving the low temperature activity of lean NOx trap (LNT) catalysts. |
WOS标题词 | Science & Technology ; Physical Sciences |
类目[WOS] | Chemistry, Physical |
研究领域[WOS] | Chemistry |
关键词[WOS] | BARRIER DISCHARGE REACTOR ; TRAP CATALYSTS ; FTIR SPECTROSCOPY ; ROOM-TEMPERATURE ; ADSORPTION ; CO ; FORMALDEHYDE ; REMOVAL ; PT/BAO/AL2O3 ; OXIDATION |
收录类别 | SCI |
语种 | 英语 |
WOS记录号 | WOS:000392399900013 |
源URL | [http://cas-ir.dicp.ac.cn/handle/321008/151864] ![]() |
专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
作者单位 | 1.Dalian Univ Technol, Sch Chem, State Key Lab Fine Chem, Dalian, Peoples R China 2.Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian, Peoples R China 3.Univ Kentucky, Ctr Appl Energy Res, Lexington, KY 40511 USA 4.Qufu Normal Univ, Sch Chem & Chem Engn, Qufu, Peoples R China |
推荐引用方式 GB/T 7714 | Li, Ming-run,Crocker, Mark,Zhang, Zhao-shun,et al. Low-temperature H-2-plasma-assisted NOx storage and reduction over a combined Pt/Ba/Al and LaMnFe catalyst[J]. CATALYSIS SCIENCE & TECHNOLOGY,2017,7(1):145-158. |
APA | Li, Ming-run,Crocker, Mark,Zhang, Zhao-shun,Shi, Chuan,Bai, Zhi-feng,&Chen, Bing-bing.(2017).Low-temperature H-2-plasma-assisted NOx storage and reduction over a combined Pt/Ba/Al and LaMnFe catalyst.CATALYSIS SCIENCE & TECHNOLOGY,7(1),145-158. |
MLA | Li, Ming-run,et al."Low-temperature H-2-plasma-assisted NOx storage and reduction over a combined Pt/Ba/Al and LaMnFe catalyst".CATALYSIS SCIENCE & TECHNOLOGY 7.1(2017):145-158. |
入库方式: OAI收割
来源:大连化学物理研究所
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