Directly converting CO2 into a gasoline fuel
文献类型：期刊论文
| 作者 | Sun, Jian1; Wei, Jian1,2; Ge, Qingjie1; Yao, Ruwei1,2; Wen, Zhiyong1,2; Fang, Chuanyan1; Guo, Lisheng1,2; Xu, Hengyong1 |
| 刊名 | NATURE COMMUNICATIONS
 |
| 出版日期 | 2017-05-02 |
| 卷号 | 8 |
| 英文摘要 | The direct production of liquid fuels from CO2 hydrogenation has attracted enormous interest for its significant roles in mitigating CO2 emissions and reducing dependence on petrochemicals. Here we report a highly efficient, stable and multifunctional Na-Fe3O4/HZSM-5 catalyst, which can directly convert CO2 to gasoline-range (C-5-C-11) hydrocarbons with selectivity up to 78% of all hydrocarbons while only 4% methane at a CO2 conversion of 22% under industrial relevant conditions. It is achieved by a multifunctional catalyst providing three types of active sites (Fe3O4, Fe5C2 and acid sites), which cooperatively catalyse a tandem reaction. More significantly, the appropriate proximity of three types of active sites plays a crucial role in the successive and synergetic catalytic conversion of CO2 to gasoline. The multifunctional catalyst, exhibiting a remarkable stability for 1,000 h on stream, definitely has the potential to be a promising industrial catalyst for CO2 utilization to liquid fuels. |
| WOS标题词 | Science & Technology |
| 类目[WOS] | Multidisciplinary Sciences |
| 研究领域[WOS] | Science & Technology - Other Topics |
| 关键词[WOS] | CARBON-DIOXIDE REDUCTION ; FISCHER-TROPSCH SYNTHESIS ; SELECTIVE CONVERSION ; METHANOL SYNTHESIS ; LOWER OLEFINS ; LIGHT OLEFINS ; CATALYSTS ; HYDROGENATION ; IRON ; ZEOLITE |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000400447700001 |
| 源URL | [http://cas-ir.dicp.ac.cn/handle/321008/151958]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 作者单位 | 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Sun, Jian,Wei, Jian,Ge, Qingjie,et al. Directly converting CO2 into a gasoline fuel[J]. NATURE COMMUNICATIONS,2017,8. |
| APA | Sun, Jian.,Wei, Jian.,Ge, Qingjie.,Yao, Ruwei.,Wen, Zhiyong.,...&Xu, Hengyong.(2017).Directly converting CO2 into a gasoline fuel.NATURE COMMUNICATIONS,8. |
| MLA | Sun, Jian,et al."Directly converting CO2 into a gasoline fuel".NATURE COMMUNICATIONS 8(2017). |
入库方式： OAI收割
来源：大连化学物理研究所
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