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  2. 合肥物质科学研究院
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  4. 中科院等离子体物理研究所
Self-templated synthesis of novel carbon nanoarchitectures for efficient electrocatalysis

文献类型：期刊论文

作者Wu, Xi-Lin1,2,3,4; Wen, Tao2,5; Guo, Hong-Li1; Liu, Shoujie1; Wang, Xiangke2,5; Xu, An-Wu1; Mezger, Markus4,6
刊名SCIENTIFIC REPORTS
出版日期2016-06-15
卷号6期号:无页码:28049
DOI10.1038/srep28049
文献子类Article
英文摘要The cost-efficient large-scale production of novel carbon nanostructure with high performance is still a challenge, restricting their applications in catalysis. Herein, we present a low-cost one-pot and one-step approach for the synthesis of both N-doped graphene (NG) and N-doped carbon nanotubes (NCNTs) from self-templated organic nanoplates. By varying the FeCl3 concentration in the precursor, we can control the formation of graphene or CNTs. To the best of our knowledge, this is the first example for the controllable synthesis of graphene or CNTs by varying the precursors' compositions. This provides a simple and cost-effective route for the large-scale production of both NG and NCNTs for applications in catalysis. By example, we show how these unique structured nanocarbons can be applied in electrocatalysis for oxygen reduction reaction (ORR). The obtained NG and NCNTs show excellent ORR activities with long-term stability under alkaline conditions. The unique porous nanostructure, abundant defects, homogeneous N-doping and high N-content in the NG and NCNTs can provide abundant active sites, leading to the excellent ORR performance. This research not only displayed a simple and cost-effective approach for the large-scale production of novel carbon nanoarchitectures, but also revealed the exceptional application potential of these nanocarbons for electrocatalysis.
WOS关键词OXYGEN REDUCTION REACTION ; GRAPHENE ; NANOTUBES ; PERFORMANCE ; ALKALINE ; SULFUR
WOS研究方向Science & Technology - Other Topics
语种英语
WOS记录号WOS:000384605400001
资助机构National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Basic Research Program of China(2011CB933700) ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; National Natural Science Foundation of China(21271165 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202) ; 91326202)
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/21878]  
专题合肥物质科学研究院_中科院等离子体物理研究所
作者单位1.Univ Sci & Technol China, Sch Nucl Sci & Technol, Div Nanomat & Chem, Hefei 230026, Peoples R China
2.North China Elect Power Univ, Sch Environm & Chem Engn, Beijing 102206, Peoples R China
3.Zhejiang Normal Univ, Coll Geog & Environm Sci, Jinhua 321004, Peoples R China
4.Max Plank Inst Polymer Res, Ackermannweg 10, D-55128 Mainz, Germany
5.Chinese Acad Sci, Inst Plasma Phys, Key Lab Novel Thin Film Solar Cells, Hefei 230031, Peoples R China
6.Johannes Gutenberg Univ Mainz, Inst Phys, D-55128 Mainz, Germany
推荐引用方式
GB/T 7714		 Wu, Xi-Lin,Wen, Tao,Guo, Hong-Li,et al. Self-templated synthesis of novel carbon nanoarchitectures for efficient electrocatalysis[J]. SCIENTIFIC REPORTS,2016,6(无):28049.
APA Wu, Xi-Lin.,Wen, Tao.,Guo, Hong-Li.,Liu, Shoujie.,Wang, Xiangke.,...&Mezger, Markus.(2016).Self-templated synthesis of novel carbon nanoarchitectures for efficient electrocatalysis.SCIENTIFIC REPORTS,6(无),28049.
MLA Wu, Xi-Lin,et al."Self-templated synthesis of novel carbon nanoarchitectures for efficient electrocatalysis".SCIENTIFIC REPORTS 6.无(2016):28049.

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来源：合肥物质科学研究院

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