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High-quality CH3NH3PbI3 thin film fabricated via intramolecular exchange for efficient planar heterojunction perovskite solar cells

文献类型：期刊论文

作者Li, Shuigen1,2; Yang, Bingchu1; Wu, Runsheng1,2; Zhang, Chen1; Zhang, Chujun1; Tang, Xiao-Fang3,4; Liu, Gang1; Liu, Peng1; Zhou, Conghua1; Gao, Yongli1,5
刊名ORGANIC ELECTRONICS
出版日期2016-12-01
卷号39期号:无页码:304-310
关键词Planar Heterojunction Perovskite Solar Cells Intramolecular Exchange Ch3nh3pbi3 Thin Film Pbi2(Dmso)
DOI10.1016/j.orgel.2016.10.017
文献子类Article
英文摘要The high-quality CH3NH3PbI3 perovskite thin film with excellent coverage and uniformity was prepared using an intramolecular exchange technology via a low-temperature, two-step sequential deposition process. The PbI2(DMSO) complex was synthesized at room temperature without any additives and was deposited, then the CH3NH3I solution was deposited subsequently. The further controllable thermal annealing process resulted in the complete formation of flat and uniform CH3NH3PbI3 thin film with large-size grains and (110) preferred crystallographic orientation. The perovskite solar cells (PSCs) with a very simple inverted planar heterojunction structure of ITO/PEDOT:PSS/CH3NH3PbI3/PCBM/Al and without other buffer layers, e.g., C-60, LiF, BCP, etc., were fabricated, resulting in a power conversion efficiency (PCE) as high as 14.26%. The results suggest that the low-temperature, two-step sequential deposition process with intramolecular exchange technology provides a good route to fabricate high quality perovskite thin film and efficient PSCs, which would match with large-scale, high-output roll to-roll (R2R) printing/coating techniques. (C) 2016 Elsevier B.V. All rights reserved.
WOS关键词ORGANOMETAL HALIDE PEROVSKITES ; HOLE-CONDUCTOR-FREE ; DEVICE EFFICIENCY ; LAYERS ; ENHANCEMENT ; DEPOSITION ; MORPHOLOGY ; ELECTRODE ; EVOLUTION
WOS研究方向Materials Science ; Physics
语种英语
WOS记录号WOS:000389087400042
资助机构China 1000-Young Talents Plan ; China 1000-Young Talents Plan ; China 1000-Young Talents Plan ; China 1000-Young Talents Plan ; China 1000-Young Talents Plan ; China 1000-Young Talents Plan ; China 1000-Young Talents Plan ; China 1000-Young Talents Plan ; National Natural Science Foundation of China(51203192 ; National Natural Science Foundation of China(51203192 ; National Natural Science Foundation of China(51203192 ; National Natural Science Foundation of China(51203192 ; National Natural Science Foundation of China(51203192 ; National Natural Science Foundation of China(51203192 ; National Natural Science Foundation of China(51203192 ; National Natural Science Foundation of China(51203192 ; Program for New Century Excellent Talents in University(NCET-13-0598) ; Program for New Century Excellent Talents in University(NCET-13-0598) ; Program for New Century Excellent Talents in University(NCET-13-0598) ; Program for New Century Excellent Talents in University(NCET-13-0598) ; Program for New Century Excellent Talents in University(NCET-13-0598) ; Program for New Century Excellent Talents in University(NCET-13-0598) ; Program for New Century Excellent Talents in University(NCET-13-0598) ; Program for New Century Excellent Talents in University(NCET-13-0598) ; Hunan Provincial Natural Science Foundation of China(2015JJ1015) ; Hunan Provincial Natural Science Foundation of China(2015JJ1015) ; Hunan Provincial Natural Science Foundation of China(2015JJ1015) ; Hunan Provincial Natural Science Foundation of China(2015JJ1015) ; Hunan Provincial Natural Science Foundation of China(2015JJ1015) ; Hunan Provincial Natural Science Foundation of China(2015JJ1015) ; Hunan Provincial Natural Science Foundation of China(2015JJ1015) ; Hunan Provincial Natural Science Foundation of China(2015JJ1015) ; Project of Innovation-driven Plan in Central South University(2015CXS036) ; Project of Innovation-driven Plan in Central South University(2015CXS036) ; Project of Innovation-driven Plan in Central South University(2015CXS036) ; Project of Innovation-driven Plan in Central South University(2015CXS036) ; Project of Innovation-driven Plan in Central South University(2015CXS036) ; Project of Innovation-driven Plan in Central South University(2015CXS036) ; Project of Innovation-driven Plan in Central South University(2015CXS036) ; Project of Innovation-driven Plan in Central South University(2015CXS036) ; National Science Foundation(DMR-1303742 ; National Science Foundation(DMR-1303742 ; National Science Foundation(DMR-1303742 ; National Science Foundation(DMR-1303742 ; National Science Foundation(DMR-1303742 ; National Science Foundation(DMR-1303742 ; National Science Foundation(DMR-1303742 ; National Science Foundation(DMR-1303742 ; 61172047 ; 61172047 ; 61172047 ; 61172047 ; 61172047 ; 61172047 ; 61172047 ; 61172047 ; CBET-1437656) ; CBET-1437656) ; CBET-1437656) ; CBET-1437656) ; CBET-1437656) ; CBET-1437656) ; CBET-1437656) ; CBET-1437656) ; 51462035 ; 51462035 ; 51462035 ; 51462035 ; 51462035 ; 51462035 ; 51462035 ; 51462035 ; 51673214) ; 51673214) ; 51673214) ; 51673214) ; 51673214) ; 51673214) ; 51673214) ; 51673214) ; China 1000-Young Talents Plan ; China 1000-Young Talents Plan ; China 1000-Young Talents Plan ; China 1000-Young Talents Plan ; China 1000-Young Talents Plan ; China 1000-Young Talents Plan ; China 1000-Young Talents Plan ; China 1000-Young Talents Plan ; National Natural Science Foundation of China(51203192 ; National Natural Science Foundation of China(51203192 ; National Natural Science Foundation of China(51203192 ; National Natural Science Foundation of China(51203192 ; National Natural Science Foundation of China(51203192 ; National Natural Science Foundation of China(51203192 ; National Natural Science Foundation of China(51203192 ; National Natural Science Foundation of China(51203192 ; Program for New Century Excellent Talents in University(NCET-13-0598) ; Program for New Century Excellent Talents in University(NCET-13-0598) ; Program for New Century Excellent Talents in University(NCET-13-0598) ; Program for New Century Excellent Talents in University(NCET-13-0598) ; Program for New Century Excellent Talents in University(NCET-13-0598) ; Program for New Century Excellent Talents in University(NCET-13-0598) ; Program for New Century Excellent Talents in University(NCET-13-0598) ; Program for New Century Excellent Talents in University(NCET-13-0598) ; Hunan Provincial Natural Science Foundation of China(2015JJ1015) ; Hunan Provincial Natural Science Foundation of China(2015JJ1015) ; Hunan Provincial Natural Science Foundation of China(2015JJ1015) ; Hunan Provincial Natural Science Foundation of China(2015JJ1015) ; Hunan Provincial Natural Science Foundation of China(2015JJ1015) ; Hunan Provincial Natural Science Foundation of China(2015JJ1015) ; Hunan Provincial Natural Science Foundation of China(2015JJ1015) ; Hunan Provincial Natural Science Foundation of China(2015JJ1015) ; Project of Innovation-driven Plan in Central South University(2015CXS036) ; Project of Innovation-driven Plan in Central South University(2015CXS036) ; Project of Innovation-driven Plan in Central South University(2015CXS036) ; Project of Innovation-driven Plan in Central South University(2015CXS036) ; Project of Innovation-driven Plan in Central South University(2015CXS036) ; Project of Innovation-driven Plan in Central South University(2015CXS036) ; Project of Innovation-driven Plan in Central South University(2015CXS036) ; Project of Innovation-driven Plan in Central South University(2015CXS036) ; National Science Foundation(DMR-1303742 ; National Science Foundation(DMR-1303742 ; National Science Foundation(DMR-1303742 ; National Science Foundation(DMR-1303742 ; National Science Foundation(DMR-1303742 ; National Science Foundation(DMR-1303742 ; National Science Foundation(DMR-1303742 ; National Science Foundation(DMR-1303742 ; 61172047 ; 61172047 ; 61172047 ; 61172047 ; 61172047 ; 61172047 ; 61172047 ; 61172047 ; CBET-1437656) ; CBET-1437656) ; CBET-1437656) ; CBET-1437656) ; CBET-1437656) ; CBET-1437656) ; CBET-1437656) ; CBET-1437656) ; 51462035 ; 51462035 ; 51462035 ; 51462035 ; 51462035 ; 51462035 ; 51462035 ; 51462035 ; 51673214) ; 51673214) ; 51673214) ; 51673214) ; 51673214) ; 51673214) ; 51673214) ; 51673214)
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/22097]  
专题合肥物质科学研究院_中科院固体物理研究所
作者单位1.Cent S Univ, Sch Phys & Elect, Hunan Key Lab Super Microstruct & Ultrafast Proc, Changsha 410083, Hunan, Peoples R China
2.Xinyu Univ, Sch New Energy Sci & Engn, Xinyu 338004, Peoples R China
3.Chinese Acad Sci, Inst Solid State Phys, Hefei 230031, Anhui, Peoples R China
4.Hunan Univ Sci & Technol, Sch Phys & Elect Sci, Xiangtan 411201, Hunan, Peoples R China
5.Univ Rochester, Dept Phys & Astron, Rochester, NY 14627 USA
6.Hunan Normal Univ, Synerget Innovat Ctr Quantum Effects & Applicat S, Changsha 410081, Hunan, Peoples R China
推荐引用方式
GB/T 7714		 Li, Shuigen,Yang, Bingchu,Wu, Runsheng,et al. High-quality CH3NH3PbI3 thin film fabricated via intramolecular exchange for efficient planar heterojunction perovskite solar cells[J]. ORGANIC ELECTRONICS,2016,39(无):304-310.
APA Li, Shuigen.,Yang, Bingchu.,Wu, Runsheng.,Zhang, Chen.,Zhang, Chujun.,...&Yang, Junliang.(2016).High-quality CH3NH3PbI3 thin film fabricated via intramolecular exchange for efficient planar heterojunction perovskite solar cells.ORGANIC ELECTRONICS,39(无),304-310.
MLA Li, Shuigen,et al."High-quality CH3NH3PbI3 thin film fabricated via intramolecular exchange for efficient planar heterojunction perovskite solar cells".ORGANIC ELECTRONICS 39.无(2016):304-310.

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来源：合肥物质科学研究院

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