Oxygen-Vacancy-Induced Antiferromagnetism to Ferromagnetism Transformation in Eu0.5Ba0.5TiO3-delta Multiferroic Thin Films
文献类型:期刊论文
作者 | Li, Weiwei1; Zhao, Run1; Wang, Le2,3; Tang, Rujun1; Zhu, Yuanyuan4; Lee, Joo Hwan4; Cao, Haixia1; Cai, Tianyi1; Guo, Haizhong2,3; Wang, Can2,3 |
刊名 | SCIENTIFIC REPORTS |
出版日期 | 2013-09-10 |
卷号 | 3 |
DOI | 10.1038/srep02618 |
文献子类 | Article |
英文摘要 | Oxygen vacancies (V-O) effects on magnetic ordering in Eu0.5Ba0.5TiO3-delta (EBTO3-delta) thin films have been investigated using a combination of experimental measurements and first-principles density-functional calculations. Two kinds of EBTO3-delta thin films with different oxygen deficiency have been fabricated. A nuclear resonance backscattering spectrometry technique has been used to quantitatively measure contents of the V-O. Eu0.5Ba0.5TiO3 ceramics have been known to exhibit ferroelectric (FE) and G-type antiferromagnetic (AFM) properties. While, a ferromagnetic (FM) behavior with a Curie temperature of 1.85 K has been found in the EBTO3-delta thin films. Spin-polarized Ti3+ ions, which originated from the V-O, has been proven to mediate a FM coupling between the local Eu 4f spins and were believed to be responsible for the great change of the magnetic ordering. Considering the easy formation of V-O, our work opens up a new avenue for achieving co-existence of FM and FE orders in oxide materials. |
WOS关键词 | INDUCED MAGNETISM ; SEMICONDUCTORS ; SPECTRA ; SRTIO3 ; OXIDE ; SIMULATION ; ELECTRON ; BATIO3 |
WOS研究方向 | Science & Technology - Other Topics |
语种 | 英语 |
WOS记录号 | WOS:000324090600001 |
源URL | [http://ir.hfcas.ac.cn:8080/handle/334002/22194] |
专题 | 合肥物质科学研究院_中科院强磁场科学中心 |
作者单位 | 1.Soochow Univ, Sch Phys Sci & Technol, Jiangsu Key Lab Thin Films, Suzhou 215006, Peoples R China 2.Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China 3.Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China 4.Texas A&M Univ, Dept Elect & Comp Engn, Mat Sci & Engn Program, College Stn, TX 77843 USA 5.Chinese Acad Sci, High Field Magnet Lab, Hefei 230031, Peoples R China 6.Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA |
推荐引用方式 GB/T 7714 | Li, Weiwei,Zhao, Run,Wang, Le,et al. Oxygen-Vacancy-Induced Antiferromagnetism to Ferromagnetism Transformation in Eu0.5Ba0.5TiO3-delta Multiferroic Thin Films[J]. SCIENTIFIC REPORTS,2013,3. |
APA | Li, Weiwei.,Zhao, Run.,Wang, Le.,Tang, Rujun.,Zhu, Yuanyuan.,...&Yang, Hao.(2013).Oxygen-Vacancy-Induced Antiferromagnetism to Ferromagnetism Transformation in Eu0.5Ba0.5TiO3-delta Multiferroic Thin Films.SCIENTIFIC REPORTS,3. |
MLA | Li, Weiwei,et al."Oxygen-Vacancy-Induced Antiferromagnetism to Ferromagnetism Transformation in Eu0.5Ba0.5TiO3-delta Multiferroic Thin Films".SCIENTIFIC REPORTS 3(2013). |
入库方式: OAI收割
来源:合肥物质科学研究院
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