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Insecticide as a precursor to prepare highly bright carbon dots for patterns printing and bioimaging: A new pathway for making poison profitable

文献类型：期刊论文

作者Zou, Wen-Sheng1,2,3; Ji, Ya-Jun1,2; Wang, Xiu-Fang1,2; Zhao, Qing-Chun1,2; Zhang, Jun1,2; Shao, Qun1,2; Liu, Jin1,2; Wang, Feng1,2; Wang, Ya-Qin1,2
刊名CHEMICAL ENGINEERING JOURNAL
出版日期2016-06-15
卷号294期号:无页码:323-332
关键词3-bromophenol Insecticide Residuals Carbon Dots Patterns Printing Bioimaging
DOI10.1016/j.cej.2016.03.004
文献子类Article
英文摘要Halophenols (HPs) inflict adverse impacts on human and environment due to their toxic, carcinogenic as well as teratogenic properties. Additionally, it is of great importance and urgency for the development of simple, efficient and inexpensive approaches to minimize the harm of HPs. Here we report an innovatively making poison profitable method to prepare carbon dots (C-dots) using 3-bromophenol residual as a precursor. The effects of solvent and carbonization temperature on the preparation of insecticide based C-dots were investigated. The results indicate that higher organic solvent content in solution and higher carbonization temperature are in favor of the formation of C-dots with smaller size and higher quantum yields. Meanwhile, all C-dots displayed excellent water solubility and high photostability against ionic strengths and light illumination. The possible mechanisms of polymerization and carbonization of C-dots were rationally proposed, and the incompact framework structure of C-dots was reasonably inferred by room-temperature phosphorescence measurement. Also, a kind of low toxicity, good biocompatibility and photostability C-dots, which were synthesized via a lab-leveled mimetic insecticide residuals approach, were utilized as colorless inks for printing patterns and as fluorescence probe for bioimaging. This proposed approach opened up a potential prospect to efficiently utilize pesticide residuals and other hazardous chemicals for biolabeling and bioimaging. (C) 2016 Elsevier B.V. All rights reserved.
WOS关键词GRAPHENE QUANTUM DOTS ; TUNABLE LUMINESCENCE PROPERTIES ; ONE-STEP SYNTHESIS ; PHOTOCATALYTIC ACTIVITY ; GREEN SYNTHESIS ; NITROGEN ; CELLS ; 2,4,6-TRICHLOROPHENOL ; PHOTOLUMINESCENCE ; NANODOTS
WOS研究方向Engineering
语种英语
WOS记录号WOS:000375170200035
资助机构Natural Science Foundation of China(21506002 ; Natural Science Foundation of China(21506002 ; Natural Science Foundation of China(21506002 ; Natural Science Foundation of China(21506002 ; Natural Science Foundation of China(21506002 ; Natural Science Foundation of China(21506002 ; Natural Science Foundation of China(21506002 ; Natural Science Foundation of China(21506002 ; Natural Science Foundation of Anhui Province(1408085MB27 ; Natural Science Foundation of Anhui Province(1408085MB27 ; Natural Science Foundation of Anhui Province(1408085MB27 ; Natural Science Foundation of Anhui Province(1408085MB27 ; Natural Science Foundation of Anhui Province(1408085MB27 ; Natural Science Foundation of Anhui Province(1408085MB27 ; Natural Science Foundation of Anhui Province(1408085MB27 ; Natural Science Foundation of Anhui Province(1408085MB27 ; Postdoctor Foundation(2013M530301) ; Postdoctor Foundation(2013M530301) ; Postdoctor Foundation(2013M530301) ; Postdoctor Foundation(2013M530301) ; Postdoctor Foundation(2013M530301) ; Postdoctor Foundation(2013M530301) ; Postdoctor Foundation(2013M530301) ; Postdoctor Foundation(2013M530301) ; 21301004 ; 21301004 ; 21301004 ; 21301004 ; 21301004 ; 21301004 ; 21301004 ; 21301004 ; 1308085MB29) ; 1308085MB29) ; 1308085MB29) ; 1308085MB29) ; 1308085MB29) ; 1308085MB29) ; 1308085MB29) ; 1308085MB29) ; 21171004) ; 21171004) ; 21171004) ; 21171004) ; 21171004) ; 21171004) ; 21171004) ; 21171004) ; Natural Science Foundation of China(21506002 ; Natural Science Foundation of China(21506002 ; Natural Science Foundation of China(21506002 ; Natural Science Foundation of China(21506002 ; Natural Science Foundation of China(21506002 ; Natural Science Foundation of China(21506002 ; Natural Science Foundation of China(21506002 ; Natural Science Foundation of China(21506002 ; Natural Science Foundation of Anhui Province(1408085MB27 ; Natural Science Foundation of Anhui Province(1408085MB27 ; Natural Science Foundation of Anhui Province(1408085MB27 ; Natural Science Foundation of Anhui Province(1408085MB27 ; Natural Science Foundation of Anhui Province(1408085MB27 ; Natural Science Foundation of Anhui Province(1408085MB27 ; Natural Science Foundation of Anhui Province(1408085MB27 ; Natural Science Foundation of Anhui Province(1408085MB27 ; Postdoctor Foundation(2013M530301) ; Postdoctor Foundation(2013M530301) ; Postdoctor Foundation(2013M530301) ; Postdoctor Foundation(2013M530301) ; Postdoctor Foundation(2013M530301) ; Postdoctor Foundation(2013M530301) ; Postdoctor Foundation(2013M530301) ; Postdoctor Foundation(2013M530301) ; 21301004 ; 21301004 ; 21301004 ; 21301004 ; 21301004 ; 21301004 ; 21301004 ; 21301004 ; 1308085MB29) ; 1308085MB29) ; 1308085MB29) ; 1308085MB29) ; 1308085MB29) ; 1308085MB29) ; 1308085MB29) ; 1308085MB29) ; 21171004) ; 21171004) ; 21171004) ; 21171004) ; 21171004) ; 21171004) ; 21171004) ; 21171004)
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/30893]  
专题合肥物质科学研究院_中科院合肥智能机械研究所
作者单位1.Anhui Jianzhu Univ, Anhui Key Lab Adv Bldg Mat, 856 South Jinzhai Rd, Hefei 230022, Anhui, Peoples R China
2.Anhui Jianzhu Univ, Key Lab Funct Mol Design & Interface Proc, 856 South Jinzhai Rd, Hefei 230022, Anhui, Peoples R China
3.Chinese Acad Sci, Inst Intelligent Machines, Hefei 230031, Anhui, Peoples R China
推荐引用方式
GB/T 7714		 Zou, Wen-Sheng,Ji, Ya-Jun,Wang, Xiu-Fang,et al. Insecticide as a precursor to prepare highly bright carbon dots for patterns printing and bioimaging: A new pathway for making poison profitable[J]. CHEMICAL ENGINEERING JOURNAL,2016,294(无):323-332.
APA Zou, Wen-Sheng.,Ji, Ya-Jun.,Wang, Xiu-Fang.,Zhao, Qing-Chun.,Zhang, Jun.,...&Wang, Ya-Qin.(2016).Insecticide as a precursor to prepare highly bright carbon dots for patterns printing and bioimaging: A new pathway for making poison profitable.CHEMICAL ENGINEERING JOURNAL,294(无),323-332.
MLA Zou, Wen-Sheng,et al."Insecticide as a precursor to prepare highly bright carbon dots for patterns printing and bioimaging: A new pathway for making poison profitable".CHEMICAL ENGINEERING JOURNAL 294.无(2016):323-332.

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来源：合肥物质科学研究院

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