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Self -assembled Pd/CeO2 catalysts by a facile redox approach for high-efficiency hydrogenation of levulinic acid into gamma-valerolactone

文献类型：期刊论文

作者Zhang, Yong1,2; Chen, Chun1; Gong, Wanbing1,2; Song, Jieyao1,2; Zhang, Haimin1; Zhang, Yunxia1; Wang, Guozhong1; Zhao, Huijun1,3
刊名CATALYSIS COMMUNICATIONS
出版日期2017-04-01
卷号93期号:无页码:10-14
关键词Pd/ceo2 Catalysts One-pot Redox Method Hydrogenation Levulinic Acid Gamma-valerolactone
DOI10.1016/j.catcom.2017.01.008
文献子类Article
英文摘要A series of self-assembled Pd/CeO2 catalysts were synthesized by a facile one-pot redox method, demonstrating high catalytic performance in hydrogenation of levulinic add. Under optimized conditions, almost 100% gammavalerolactone yield was achieved using Pd/CeO2 catalyst with only slight activity loss (ca. 4%) after five continuous runs. Combined with relevant characterization techniques, the superior catalytic hydrogenation performance could be attributed to Pd/CeO2 catalyst with noticeable advantages of high surface area beneficial to the exposure of Pd catalytic active sites and increase electron density of Pd favorable for the dissociation of H-2 as well as the defects sites of CeO2 responsible for esterification of intermediate. (C) 2017 Elsevier B.V. All rights reserved.
WOS关键词SELECTIVE PRODUCTION ; PHASE HYDROGENATION ; BIOMASS ; CHEMICALS ; FUELS ; CERIA ; TRANSFORMATION ; DEHYDRATION ; PLATFORM ; SUPPORT
WOS研究方向Chemistry
语种英语
WOS记录号WOS:000397685600003
资助机构National Natural Science Foundation of China(51372248 ; National Natural Science Foundation of China(51372248 ; National Natural Science Foundation of China(51372248 ; National Natural Science Foundation of China(51372248 ; CAS/SAFEA International Partnership Program for Creative Research Teams of Chinese Academy of Sciences, China ; CAS/SAFEA International Partnership Program for Creative Research Teams of Chinese Academy of Sciences, China ; CAS/SAFEA International Partnership Program for Creative Research Teams of Chinese Academy of Sciences, China ; CAS/SAFEA International Partnership Program for Creative Research Teams of Chinese Academy of Sciences, China ; CAS Pioneer Hundred Talents Program, and the Users of Potential Program(2015HSC-UP006) ; CAS Pioneer Hundred Talents Program, and the Users of Potential Program(2015HSC-UP006) ; CAS Pioneer Hundred Talents Program, and the Users of Potential Program(2015HSC-UP006) ; CAS Pioneer Hundred Talents Program, and the Users of Potential Program(2015HSC-UP006) ; 51432009 ; 51432009 ; 51432009 ; 51432009 ; 51502297) ; 51502297) ; 51502297) ; 51502297) ; National Natural Science Foundation of China(51372248 ; National Natural Science Foundation of China(51372248 ; National Natural Science Foundation of China(51372248 ; National Natural Science Foundation of China(51372248 ; CAS/SAFEA International Partnership Program for Creative Research Teams of Chinese Academy of Sciences, China ; CAS/SAFEA International Partnership Program for Creative Research Teams of Chinese Academy of Sciences, China ; CAS/SAFEA International Partnership Program for Creative Research Teams of Chinese Academy of Sciences, China ; CAS/SAFEA International Partnership Program for Creative Research Teams of Chinese Academy of Sciences, China ; CAS Pioneer Hundred Talents Program, and the Users of Potential Program(2015HSC-UP006) ; CAS Pioneer Hundred Talents Program, and the Users of Potential Program(2015HSC-UP006) ; CAS Pioneer Hundred Talents Program, and the Users of Potential Program(2015HSC-UP006) ; CAS Pioneer Hundred Talents Program, and the Users of Potential Program(2015HSC-UP006) ; 51432009 ; 51432009 ; 51432009 ; 51432009 ; 51502297) ; 51502297) ; 51502297) ; 51502297)
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/32944]  
专题合肥物质科学研究院_中科院固体物理研究所
作者单位1.Chinese Acad Sci, Key Lab Mat Phys, Ctr Environm & Energy Nanomat,Inst Solid State Ph, Anhui Key Lab Nanomat & Nanotechnol,CAS Ctr Excel, Hefei 230031, Peoples R China
2.Univ Sci & Technol China, Hefei 230026, Anhui, Peoples R China
3.Griffith Univ, Ctr Clean Environm & Energy, Gold Coast Campus, Southport, Qld 4222, Australia
推荐引用方式
GB/T 7714		 Zhang, Yong,Chen, Chun,Gong, Wanbing,et al. Self -assembled Pd/CeO2 catalysts by a facile redox approach for high-efficiency hydrogenation of levulinic acid into gamma-valerolactone[J]. CATALYSIS COMMUNICATIONS,2017,93(无):10-14.
APA Zhang, Yong.,Chen, Chun.,Gong, Wanbing.,Song, Jieyao.,Zhang, Haimin.,...&Zhao, Huijun.(2017).Self -assembled Pd/CeO2 catalysts by a facile redox approach for high-efficiency hydrogenation of levulinic acid into gamma-valerolactone.CATALYSIS COMMUNICATIONS,93(无),10-14.
MLA Zhang, Yong,et al."Self -assembled Pd/CeO2 catalysts by a facile redox approach for high-efficiency hydrogenation of levulinic acid into gamma-valerolactone".CATALYSIS COMMUNICATIONS 93.无(2017):10-14.

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来源：合肥物质科学研究院

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