Highly efficient and durable MoNiNC catalyst for hydrogen evolution reaction
文献类型：期刊论文
| 作者 | Liu, Linghui2,5; Wang, Fanan2,3; Sun, Yuanmiao6; He, Yanghua2; Xu, Jinming2; Zhao, Xiaochen2; Yin, Guangzhao1; Zhang, Liping1; Li, Shuzhou6; Mao, Qing1 |
| 刊名 | NANO ENERGY
 |
| 出版日期 | 2017-07-01 |
| 卷号 | 37页码:1-6 |
| 关键词 | Carbothermal Ammonia Reduction Electrochemical Carbonitride Hydrogen Evolution Reaction Electrocatalyst |
| DOI | 10.1016/j.nanoen.2017.04.050 |
| 英文摘要 | We report a carbothermal ammonia reduction (CAR) strategy for one-pot preparation of highly efficient and durable hydrogen evolution reaction (HER) electrocatalyst composed of earth abundant early transition metals. In this strategy, resin is applied both as the pre-binder and carbon source, and Pluronic F127 as the structuredirecting agent. Upon annealing in NH3, the Mo-containing precursor on Ni foam undergoes the CAR, and simultaneously Ni from the substrate diffuses out, resulting in the formation of a quaternary complex structure of molybdenum-nickel bimetallic carbonitride (MoNiNC). The as-prepared electrode showed outstanding HER performance with an overpotential of 150 mV at 50 mA cm(-2) and maintained steady hydrogen bubble evolution for continuous 48 h. Our strategy offers a quick and simple way to fabricate earth-abundant HER electrode with highly efficient and durable electrocatalytic performance. |
| 语种 | 英语 |
| WOS记录号 | WOS:000402704500001 |
| 源URL | [http://cas-ir.dicp.ac.cn/handle/321008/152245]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 作者单位 | 1.Dalian Univ Technol, Sch Chem Engn, 2 Linggong Rd, Dalian 116024, Peoples R China 2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, 457 Zhongshan Rd, Dalian 116023, Peoples R China 3.Univ Chinese Acad Sci, 19A Yuquan Rd, Beijing 100049, Peoples R China 4.Nanyang Technol Univ, Sch Chem & Biomed Engn, 62 Nanyang Dr, Singapore 637459, Singapore 5.Chongqing Univ, Sch Chem & Chem Engn, Shapingba 174, Chongqing 400044, Peoples R China 6.Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore |
| 推荐引用方式 GB/T 7714 | Liu, Linghui,Wang, Fanan,Sun, Yuanmiao,et al. Highly efficient and durable MoNiNC catalyst for hydrogen evolution reaction[J]. NANO ENERGY,2017,37:1-6. |
| APA | Liu, Linghui.,Wang, Fanan.,Sun, Yuanmiao.,He, Yanghua.,Xu, Jinming.,...&Liu, Bin.(2017).Highly efficient and durable MoNiNC catalyst for hydrogen evolution reaction.NANO ENERGY,37,1-6. |
| MLA | Liu, Linghui,et al."Highly efficient and durable MoNiNC catalyst for hydrogen evolution reaction".NANO ENERGY 37(2017):1-6. |
入库方式： OAI收割
来源：大连化学物理研究所
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