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Free-Standing Holey Ni(OH)(2) Nanosheets with Enhanced Activity for Water Oxidation

文献类型：期刊论文

作者Kong, Xiangkai1,2,3; Zhang, Changlin1; Hwang, Sang Youp1; Chen, Qianwang3,4; Peng, Zhenmeng1
刊名SMALL
出版日期2017-07-12
卷号13期号:26
DOI10.1002/smll.201700334
文献子类Article
英文摘要Electrochemical water oxidation is the key technology in water-splitting reactions and rechargeable metal-air batteries, which is very attractive for renewable energy conversion and storage. Replacement of precious catalysts with cost-effective and highly active alternatives is still a great challenge. Herein, based on theoretical predictions, holey structures are designed and fabricated on the free-standing conventional 2D OER catalyst. By well-controlled defects engineering, uniform tiny holes are created on the free-standing Ni(OH)(2) nanosheets via a sol-gel method, with the embedded Zn components as the template for holes production. The whole preparation process is feasible and effective to make full use of the basal plane of 2D nanomaterials, which can provide higher surface area, richer defects, more grain boundaries, and edge sites, as well as greater distorted surfaces. Meanwhile, these holes developed inside the sheet structure can supply tremendous permeable channels for ions adsorption and transportation, enable a fast interfacial charge transfer and accelerate the reaction process. The as-prepared 2D holey Ni(OH)(2) nanostructures exhibit excellent catalytic performance toward electrochemical water oxidation, with lower onset overpotentials and higher current densities compared with the pristine Ni(OH)(2) catalyst, suggesting the holey defects engineering is a promising strategy for efficient water-splitting devices and rechargeable metal-air batteries.
WOS关键词OXYGEN EVOLUTION REACTION ; HYDROGEN EVOLUTION ; NICKEL-HYDROXIDE ; AIR-BATTERIES ; CATALYSTS ; ELECTROCATALYST ; EFFICIENT ; ELECTROLYSIS ; CATHODE ; ROBUST
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
语种英语
WOS记录号WOS:000404986200009
资助机构University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; China Postdoctoral Science Foundation(2016M600492) ; 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Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; University of Akron ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; National Natural Science Foundation of China(51602116) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; China Postdoctoral Science Foundation(2016M600492) ; China Postdoctoral Science Foundation(2016M600492) ; China Postdoctoral Science Foundation(2016M600492) ; China Postdoctoral Science Foundation(2016M600492) ; China Postdoctoral Science Foundation(2016M600492) ; China Postdoctoral Science Foundation(2016M600492) ; China Postdoctoral Science Foundation(2016M600492) ; 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Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Chinese Academy of Sciences (CAS)/State Administration of Foreign Experts Affairs (SAFEA) International Partnership Program for Creative Research Teams ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011) ; Hefei Science Center CAS(2016HSC-IU011)
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/33457]  
专题合肥物质科学研究院_中科院强磁场科学中心
作者单位1.Univ Akron, Dept Chem & Biomol Engn, Akron, OH 44325 USA
2.Huaibei Normal Univ, Sch Phys & Elect Informat, Huaibei 235000, Anhui, Peoples R China
3.Chinese Acad Sci, High Field Magnet Lab, Hefei 230031, Anhui, Peoples R China
4.Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China
推荐引用方式
GB/T 7714		 Kong, Xiangkai,Zhang, Changlin,Hwang, Sang Youp,et al. Free-Standing Holey Ni(OH)(2) Nanosheets with Enhanced Activity for Water Oxidation[J]. SMALL,2017,13(26).
APA Kong, Xiangkai,Zhang, Changlin,Hwang, Sang Youp,Chen, Qianwang,&Peng, Zhenmeng.(2017).Free-Standing Holey Ni(OH)(2) Nanosheets with Enhanced Activity for Water Oxidation.SMALL,13(26).
MLA Kong, Xiangkai,et al."Free-Standing Holey Ni(OH)(2) Nanosheets with Enhanced Activity for Water Oxidation".SMALL 13.26(2017).

入库方式： OAI收割

来源：合肥物质科学研究院

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