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Synthesis of a Multifunctional Graphene Oxide-Based Magnetic Nanocomposite for Efficient Removal of Cr(VI)

文献类型：期刊论文

作者Wang, Dongfang1,3; Zhang, Guilong1,2; Zhou, Linglin1,3; Wang, Min1,3; Cai, Dongqing1,2; Wu, Zhengyan1,2
刊名LANGMUIR
出版日期2017-07-18
卷号33期号:28页码:7007-7014
DOI10.1021/acs.langmuir.7b01293
文献子类Article
英文摘要A novel magnetic nanocomposite was synthesized using graphene oxide (GO), polyethylenimine (PEI), and Fe3O4 to removal hexavalent chromium (Cr(VI)) from water and soil. Therein, GO was functionalized with plenty of -NH2 by the modification of PEI through an amidation reaction, and the resulting GO/PEI reacted with FeSO4 center dot 7H(2)O and NaBH4 to obtain RGO/PEI/Fe3O4 (the optimal one is designated as ORPF) through an oxidation- reduction reaction. ORPF could effectively adsorb Cr(VI) through electrostatic attraction, and the adsorbed Cr(VI) ions were partially reduced to trivalent chromium (Cr(III)) with low toxicity by RGO (pi electron). Afterward, the resulting ORPF-Cr could be conveniently removed from water with a magnet, achieving the maximum Cr(VI) removal capacity of 266.6 mg/g. Importantly, ORPF, once carried by sponge particles, could efficiently remove Cr(VI) from soil, and the resulting mixture could be facilely collected with a magnet on a filter net. Besides, the leaching experiment suggested that, when supported by filter paper, ORPF was able to decrease the number of leached Cr(VI) ions and meanwhile reduce them to Cr(III). This work provides a promising approach to remediate Cr(VI))-contaminated water and soil using a nanocomposite, Which has a huge number of application prospects.
WOS关键词ZERO-VALENT IRON ; AQUEOUS-SOLUTIONS ; HEXAVALENT CHROMIUM ; FACILE SYNTHESIS ; WASTE-WATER ; REDUCTION ; FABRICATION ; ADSORPTION ; ADSORBENT ; ACTIVATION
WOS研究方向Chemistry ; Materials Science
语种英语
WOS记录号WOS:000406086000007
资助机构National Natural Science Foundation of China(21407151) ; National Natural Science Foundation of China(21407151) ; National Natural Science Foundation of China(21407151) ; National Natural Science Foundation of China(21407151) ; National Natural Science Foundation of China(21407151) ; National Natural Science Foundation of China(21407151) ; National Natural Science Foundation of China(21407151) ; National Natural Science Foundation of China(21407151) ; Youth Innovation Promotion Association of the Chinese Academy of Sciences(2015385) ; Youth Innovation Promotion Association of the Chinese Academy of Sciences(2015385) ; Youth Innovation Promotion Association of the Chinese Academy of Sciences(2015385) ; Youth Innovation Promotion Association of the Chinese Academy of Sciences(2015385) ; Youth Innovation Promotion Association of the Chinese Academy of Sciences(2015385) ; Youth Innovation Promotion Association of the Chinese Academy of Sciences(2015385) ; Youth Innovation Promotion Association of the Chinese Academy of Sciences(2015385) ; Youth Innovation Promotion Association of the Chinese Academy of Sciences(2015385) ; Key Program of the Chinese Academy of Sciences(KSZD-EW-Z-022-05) ; Key Program of the Chinese Academy of Sciences(KSZD-EW-Z-022-05) ; Key Program of the Chinese Academy of Sciences(KSZD-EW-Z-022-05) ; Key Program of the Chinese Academy of Sciences(KSZD-EW-Z-022-05) ; Key Program of the Chinese Academy of Sciences(KSZD-EW-Z-022-05) ; Key Program of the Chinese Academy of Sciences(KSZD-EW-Z-022-05) ; Key Program of the Chinese Academy of Sciences(KSZD-EW-Z-022-05) ; Key Program of the Chinese Academy of Sciences(KSZD-EW-Z-022-05) ; Science and Technology Service Programs of the Chinese Academy of Sciences(KFJ-STS-ZDTP-002 ; Science and Technology Service Programs of the Chinese Academy of Sciences(KFJ-STS-ZDTP-002 ; Science and Technology Service Programs of the Chinese Academy of Sciences(KFJ-STS-ZDTP-002 ; Science and Technology Service Programs of the Chinese Academy of Sciences(KFJ-STS-ZDTP-002 ; Science and Technology Service Programs of the Chinese Academy of Sciences(KFJ-STS-ZDTP-002 ; Science and Technology Service Programs of the Chinese Academy of Sciences(KFJ-STS-ZDTP-002 ; Science and Technology Service Programs of the Chinese Academy of Sciences(KFJ-STS-ZDTP-002 ; Science and Technology Service Programs of the Chinese Academy of Sciences(KFJ-STS-ZDTP-002 ; President Foundation of Hefei Institutes of Physical Science of Chinese Academy of Sciences(YZJJ201502) ; President Foundation of Hefei Institutes of Physical Science of Chinese Academy of Sciences(YZJJ201502) ; President Foundation of Hefei Institutes of Physical Science of Chinese Academy of Sciences(YZJJ201502) ; President Foundation of Hefei Institutes of Physical Science of Chinese Academy of Sciences(YZJJ201502) ; President Foundation of Hefei Institutes of Physical Science of Chinese Academy of Sciences(YZJJ201502) ; President Foundation of Hefei Institutes of Physical Science of Chinese Academy of Sciences(YZJJ201502) ; President Foundation of Hefei Institutes of Physical Science of Chinese Academy of Sciences(YZJJ201502) ; President Foundation of Hefei Institutes of Physical Science of Chinese Academy of Sciences(YZJJ201502) ; KFJ-SWSTS-143) ; KFJ-SWSTS-143) ; KFJ-SWSTS-143) ; KFJ-SWSTS-143) ; KFJ-SWSTS-143) ; KFJ-SWSTS-143) ; KFJ-SWSTS-143) ; KFJ-SWSTS-143) ; National Natural Science Foundation of China(21407151) ; National Natural Science Foundation of China(21407151) ; National Natural Science Foundation of China(21407151) ; National Natural Science Foundation of China(21407151) ; National Natural Science Foundation of China(21407151) ; National Natural Science Foundation of China(21407151) ; National Natural Science Foundation of China(21407151) ; National Natural Science Foundation of China(21407151) ; Youth Innovation Promotion Association of the Chinese Academy of Sciences(2015385) ; Youth Innovation Promotion Association of the Chinese Academy of Sciences(2015385) ; Youth Innovation Promotion Association of the Chinese Academy of Sciences(2015385) ; Youth Innovation Promotion Association of the Chinese Academy of Sciences(2015385) ; Youth Innovation Promotion Association of the Chinese Academy of Sciences(2015385) ; Youth Innovation Promotion Association of the Chinese Academy of Sciences(2015385) ; Youth Innovation Promotion Association of the Chinese Academy of Sciences(2015385) ; Youth Innovation Promotion Association of the Chinese Academy of Sciences(2015385) ; Key Program of the Chinese Academy of Sciences(KSZD-EW-Z-022-05) ; Key Program of the Chinese Academy of Sciences(KSZD-EW-Z-022-05) ; Key Program of the Chinese Academy of Sciences(KSZD-EW-Z-022-05) ; Key Program of the Chinese Academy of Sciences(KSZD-EW-Z-022-05) ; Key Program of the Chinese Academy of Sciences(KSZD-EW-Z-022-05) ; Key Program of the Chinese Academy of Sciences(KSZD-EW-Z-022-05) ; Key Program of the Chinese Academy of Sciences(KSZD-EW-Z-022-05) ; Key Program of the Chinese Academy of Sciences(KSZD-EW-Z-022-05) ; Science and Technology Service Programs of the Chinese Academy of Sciences(KFJ-STS-ZDTP-002 ; Science and Technology Service Programs of the Chinese Academy of Sciences(KFJ-STS-ZDTP-002 ; Science and Technology Service Programs of the Chinese Academy of Sciences(KFJ-STS-ZDTP-002 ; Science and Technology Service Programs of the Chinese Academy of Sciences(KFJ-STS-ZDTP-002 ; Science and Technology Service Programs of the Chinese Academy of Sciences(KFJ-STS-ZDTP-002 ; Science and Technology Service Programs of the Chinese Academy of Sciences(KFJ-STS-ZDTP-002 ; Science and Technology Service Programs of the Chinese Academy of Sciences(KFJ-STS-ZDTP-002 ; Science and Technology Service Programs of the Chinese Academy of Sciences(KFJ-STS-ZDTP-002 ; President Foundation of Hefei Institutes of Physical Science of Chinese Academy of Sciences(YZJJ201502) ; President Foundation of Hefei Institutes of Physical Science of Chinese Academy of Sciences(YZJJ201502) ; President Foundation of Hefei Institutes of Physical Science of Chinese Academy of Sciences(YZJJ201502) ; President Foundation of Hefei Institutes of Physical Science of Chinese Academy of Sciences(YZJJ201502) ; President Foundation of Hefei Institutes of Physical Science of Chinese Academy of Sciences(YZJJ201502) ; President Foundation of Hefei Institutes of Physical Science of Chinese Academy of Sciences(YZJJ201502) ; President Foundation of Hefei Institutes of Physical Science of Chinese Academy of Sciences(YZJJ201502) ; President Foundation of Hefei Institutes of Physical Science of Chinese Academy of Sciences(YZJJ201502) ; KFJ-SWSTS-143) ; KFJ-SWSTS-143) ; KFJ-SWSTS-143) ; KFJ-SWSTS-143) ; KFJ-SWSTS-143) ; KFJ-SWSTS-143) ; KFJ-SWSTS-143) ; KFJ-SWSTS-143)
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/33531]  
专题合肥物质科学研究院_技术生物与农业工程研究所
作者单位1.Chinese Acad Sci, Hefei Inst Phys Sci, Key Lab Ion Beam Bioengn, 350 Shushanhu Rd, Hefei 230031, Anhui, Peoples R China
2.Chinese Acad Sci, Hefei Inst Phys Sci, Key Lab Environm Toxicol & Pollut Control Technol, 350 Shushanhu Rd, Hefei 230031, Anhui, Peoples R China
3.Univ Sci & Technol China, 96 Jinzhai Rd, Hefei 230026, Anhui, Peoples R China
推荐引用方式
GB/T 7714		 Wang, Dongfang,Zhang, Guilong,Zhou, Linglin,et al. Synthesis of a Multifunctional Graphene Oxide-Based Magnetic Nanocomposite for Efficient Removal of Cr(VI)[J]. LANGMUIR,2017,33(28):7007-7014.
APA Wang, Dongfang,Zhang, Guilong,Zhou, Linglin,Wang, Min,Cai, Dongqing,&Wu, Zhengyan.(2017).Synthesis of a Multifunctional Graphene Oxide-Based Magnetic Nanocomposite for Efficient Removal of Cr(VI).LANGMUIR,33(28),7007-7014.
MLA Wang, Dongfang,et al."Synthesis of a Multifunctional Graphene Oxide-Based Magnetic Nanocomposite for Efficient Removal of Cr(VI)".LANGMUIR 33.28(2017):7007-7014.

入库方式： OAI收割

来源：合肥物质科学研究院

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