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Quasi-solid-state dye-sensitized solar cell based on gel electrolyte with high gel to solution transition temperature using low molecular mass organogelator

文献类型：期刊论文

作者Wang, Lu1,2; Huo, Zhipeng1; Tao, Li4; Zhu, Jun1; Zhang, Changneng1; Chen, Shuanghong1; Dai, Songyuan1,3
刊名JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY
出版日期2016-10-01
卷号329期号:无页码:139-145
关键词Quasi-solid-state Dye-sensitized Solar Cell Electrolyte Low Molecular Mass Organogelator Stability
DOI10.1016/j.jphotochem.2016.05.027
文献子类Article
英文摘要Quasi-solid-state dye-sensitized solar cell (QS-DSSC) were fabricated using N,N'-1,4-butylenediylbis-dodecanamide as low molecular mass organogelator (LMOG). The gel to solution transition temperature (T-gel) of this gel electrolyte is 115.8 degrees C which ensures a good intrinsic stability of the gel electrolyte at the QS-DSSC operating temperature. The kinetic processes of electron transport and recombination of DSSCs influenced by the gel electrolyte are investigated in detail. Due to the diffusion of redox species in the gel electrolyte is hindered by the crosslinked network and the electron recombination at the interface of the TiO2 photoanode/electrolyte is accelerated, the incidental photon-to-electron conversion efficiency (IPCE) and the short circuit photocurrent density (J(sc)) of the QS-DSSC are slightly decreased compared with those of liquid electrolyte based DSSC (L-DSSC). Remarkably, the QS-DSSC exhibits excellent thermal and light-soaking stabilities during accelerated aging tests for 1000 h. The QS-DSSC retains 90% of its initial photoelectric conversion efficiency, whereas that of L-DSSC only retains 83% under successive one sun light soaking with UV cut-off filter at 50 degrees C for 1000 h. (C) 2016 Elsevier B.V. All rights reserved.
WOS关键词NANOCRYSTALLINE TIO2 ; HIGH-EFFICIENCY ; POLYMER ELECTROLYTE ; CHARGE-TRANSPORT ; ADSORBED CATIONS ; HOLE CONDUCTOR ; RECOMBINATION ; DERIVATIVES ; CONVERSION ; INTERFACE
WOS研究方向Chemistry
语种英语
WOS记录号WOS:000381837500017
资助机构National High Technology Research and Development Program of China(2015AA050602) ; National High Technology Research and Development Program of China(2015AA050602) ; National High Technology Research and Development Program of China(2015AA050602) ; National High Technology Research and Development Program of China(2015AA050602) ; National Natural Science Foundation of China(21103197 ; National Natural Science Foundation of China(21103197 ; National Natural Science Foundation of China(21103197 ; National Natural Science Foundation of China(21103197 ; National Basic Research Program of China(2015CB932200) ; National Basic Research Program of China(2015CB932200) ; National Basic Research Program of China(2015CB932200) ; National Basic Research Program of China(2015CB932200) ; project of scientific and technological support program in Jiangsu province(BE2014147-4) ; project of scientific and technological support program in Jiangsu province(BE2014147-4) ; project of scientific and technological support program in Jiangsu province(BE2014147-4) ; project of scientific and technological support program in Jiangsu province(BE2014147-4) ; Beijing Municipal Science and Technology Project(Z141100003314003) ; Beijing Municipal Science and Technology Project(Z141100003314003) ; Beijing Municipal Science and Technology Project(Z141100003314003) ; Beijing Municipal Science and Technology Project(Z141100003314003) ; 21403247 ; 21403247 ; 21403247 ; 21403247 ; 61404142 ; 61404142 ; 61404142 ; 61404142 ; 21273242) ; 21273242) ; 21273242) ; 21273242) ; National High Technology Research and Development Program of China(2015AA050602) ; National High Technology Research and Development Program of China(2015AA050602) ; National High Technology Research and Development Program of China(2015AA050602) ; National High Technology Research and Development Program of China(2015AA050602) ; National Natural Science Foundation of China(21103197 ; National Natural Science Foundation of China(21103197 ; National Natural Science Foundation of China(21103197 ; National Natural Science Foundation of China(21103197 ; National Basic Research Program of China(2015CB932200) ; National Basic Research Program of China(2015CB932200) ; National Basic Research Program of China(2015CB932200) ; National Basic Research Program of China(2015CB932200) ; project of scientific and technological support program in Jiangsu province(BE2014147-4) ; project of scientific and technological support program in Jiangsu province(BE2014147-4) ; project of scientific and technological support program in Jiangsu province(BE2014147-4) ; project of scientific and technological support program in Jiangsu province(BE2014147-4) ; Beijing Municipal Science and Technology Project(Z141100003314003) ; Beijing Municipal Science and Technology Project(Z141100003314003) ; Beijing Municipal Science and Technology Project(Z141100003314003) ; Beijing Municipal Science and Technology Project(Z141100003314003) ; 21403247 ; 21403247 ; 21403247 ; 21403247 ; 61404142 ; 61404142 ; 61404142 ; 61404142 ; 21273242) ; 21273242) ; 21273242) ; 21273242)
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/23868]  
专题合肥物质科学研究院_应用技术研究所
作者单位1.Chinese Acad Sci, Hefei Inst Phys Sci, Inst Appl Technol, Key Lab Novel Thin Film Solar Cells, Hefei 230088, Anhui, Peoples R China
2.Univ Sci & Technol China, Hefei 230026, Anhui, Peoples R China
3.North China Elect Power Univ, Sch Renewable Energy, Beijing Key Lab Novel Thin Film Solar Cells, Beijing 102206, Peoples R China
4.Hubei Univ, Fac Phys & Elect Sci, Hubei Collaborat Innovat Ctr Adv Organ Chem Mat, Wuhan 430062, Peoples R China
推荐引用方式
GB/T 7714		 Wang, Lu,Huo, Zhipeng,Tao, Li,et al. Quasi-solid-state dye-sensitized solar cell based on gel electrolyte with high gel to solution transition temperature using low molecular mass organogelator[J]. JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY,2016,329(无):139-145.
APA Wang, Lu.,Huo, Zhipeng.,Tao, Li.,Zhu, Jun.,Zhang, Changneng.,...&Dai, Songyuan.(2016).Quasi-solid-state dye-sensitized solar cell based on gel electrolyte with high gel to solution transition temperature using low molecular mass organogelator.JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY,329(无),139-145.
MLA Wang, Lu,et al."Quasi-solid-state dye-sensitized solar cell based on gel electrolyte with high gel to solution transition temperature using low molecular mass organogelator".JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY 329.无(2016):139-145.

入库方式： OAI收割

来源：合肥物质科学研究院

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